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. Author manuscript; available in PMC: 2017 Sep 24.
Published in final edited form as: J Phys Chem B. 2016 Dec 19;120(51):13003–13016. doi: 10.1021/acs.jpcb.6b08449

Figure 3. Transition pathway contributions to 2nd- and 4th-order TCFs for two-state (N = 2) system.

Figure 3

(A) There are N2 = 22 = 4 possible outcomes of a time-ordered two-point product of the observable A(t), which are used to construct the 2nd-order TCF C̄(2)(τ). (B) There are N4 = 24 = 16 such sequences for the four-point product that is used to construct the 4th-order TCF C̄(4)(τ1, τ2, τ3). The conditional probability pji(τ) that a stochastic transition will occur from state-i to state-j within the time interval τ is given by Eq. (10).