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. Author manuscript; available in PMC: 2018 Jun 1.
Published in final edited form as: Biomaterials. 2017 Mar 15;129:54–67. doi: 10.1016/j.biomaterials.2017.03.013

Table 2.

Nucleus pulposus repair or replacement devices

Polymer Trade name or reference Clinical trials? Measurement outcomes/comments
Injectable synthetic polymers
Copolymeric hydrogel (PAN and polyacrylamide) encased in a polyethylene fiber jacket PDN Yes No longer in use
Semihydrated poly(vinyl) alcohol Aquarelle Yes No longer in use
Copolymer of poly(vinyl alcohol) [and poly(vinyl pyrrolidone) or modified PAN] reinforced by a Dacron mesh NeuDisc™ Yes Restored compressive stiffness
Hydrating PAN NucleoFix™ Yes Marketed under CE mark
In situ forming (or cross-linked) synthetic and biologically based polymers
In situ curing polymer using inflatable polyurethane “balloon” DASCOR™ Yes Restored multidirectional segment flexibility
In situ curing polymerized water-in-oil emulsion composite DiscCell™ Yes From in vitro work: restored motion segment stabilitya
Glutaraldehyde cross-linked albumin Biodisc™ Yes Uncertain status
Hydrogel of a chemically cross-linked elastin and silk polypeptide NuCore™ Yes Maintenance of disc height; significantly reduced leg and back pain; improved function scores in discectomy patients
Oxidized hyaluronic acid gelatin implant 133 Preclinical Restored motion segment stability; no changes in stiffness
Thiol-modified hyaluronan and elastin-like polypeptide 134 Preclinical Restored stiffness
Sulfonate-containing glycosaminoglycan surrogates 135 NA Restored stiffness; maintained disc height under compression
Silk fibroin/polyurethane composite 136 Preclinical Mechanical properties stable over time; higher stiffness than native NP but conducive for cell support
PNIPAAm-PEG hydrogels 137 NA Enhanced recovery from compressive strain, was thermoresponsive, sustained drug release
Chitosan gels 138 NA Supported matrix accumulation for native cells and retention of proteoglycan
Hyaluronic acid/collagen hydrogel 93 Preclinical Implant did not improve disc height; increased scarring and inflammation in AF
Hyaluronan polymers 139 Preclinical Prevented fibrotic changes; supported cell growth; no mechanical outcomes
Hyaluroan / PEG crosslinked copolymer 102 NA Engineered design that could be targeted to maintain NP or AF cell phenotype in vitro
Collagen type II / hyaluronan-PEG crosslinked hydrogel 104 NA Supported maintenance of cell phenotype and biosynthesis for native NP cells

Restored stability is equivalent to reduced range of motion in flexion—extension, lateral bending, or restored neutral zone mechanics. Abbreviations: AF, anulus fibrosus; CE, European Conformity; NP, nucleus pulposus; PAN, polyacrylonitrile; PEG, polyethylene glycol; PNIPPAm, poly(N-isopropyl acrylamide).