Table 4.
Krypton in aluminum solar wind collectors released in five different laser ablation experiments. Isotopic ratios 83Kr/84Kr, 82Kr/84Kr and 80Kr/84Kr were measured twice using different ion collectors. Comparison of these two measurements served as an internal test of multiplier performance. A small fraction of analyses rejected based on this test are not shown here. Blanks represent weighted average of several analyses. Atmospheric values are from Basford et al., 1973.
| Sample, extraction method | Area (cm2) | 84Kr, 106 at. | 86Kr/84Kr | 83Kr/84Kr | 82Kr/84Kr | 80Kr/84Kr | 78Kr/84Kr | 132Xe/84Kr | Fraction of SW 84Kr | SW 84Kr retrieved 107 at/cm2 |
|---|---|---|---|---|---|---|---|---|---|---|
| A-π/8 (a) | Blank | 0.18 | 0.3067 (95) | 0.2134(120) | 0.2022 (100) | 0.0508 (36) | 0.00605 (530) | 0.0435 | ||
| 0.2014(88) | 0.2065 (80) | 0.0494 (44) | 0.0438 | |||||||
| IR-laser ablation of Al-film on AloS. The beam hits the Al surface at 22.5° angle from normal incident. Y-stage is mounted on X-stage at 22.5° | 0.81 | 11.53 | 0.3026 (17) | 0.2018 (14) | 0.2083 (13) | 0.0404 (6) | 0.00638 (17) | 0.0953 | 0.85 | 1.21 |
| 0.2036 (13) | 0.2042 (11) | 0.0410 (7) | 0.0966 | |||||||
| 0.72 | 11.16 | 0.3039 (11) | 0.2032 (11) | 0.2022 (10) | 0.0403 (4) | 0.00632 (19) | 0.0899 | 0.77 | 1.19 | |
| 0.2027 (10) | 0.2037 (9) | 0.0391 (5) | 0.0894 | |||||||
| 0.38 | 7.26 | 0.3002 (16) | 0.2019 (13) | 0.2029 (14) | 0.0405 (6) | 0.00585 (28) | 0.0827 | 0.65 | 1.25 | |
| 0.2032 (13) | 0.2017 (12) | 0.0411 (6) | 0.0822 | |||||||
| 0.052 | 0.84 | 0.3030 (40) | 0.2026 (33) | 0.2087 (30) | 0.0432 (13) | 0.00665 (55) | 0.0863 | 0.71 | 1.15 | |
| 0.2041 (32) | 0.2065 (30) | 0.0386 (14) | 0.0856 | |||||||
| A-π/8 (b) | 0.96 | 11.82 | 0.3004 (19) | 0.2046 (19) | 0.2053 (16) | 0.0393 (6) | 0.00652 (22) | 0.1019 | 0.96 | 1.18 |
| 0.2041 (12) | 0.2042 (11) | 0.0410 (6) | 0.1026 | |||||||
| Same as A-π/8 (a) but made 5 months later under slightly different conditions | 3.82 | 50.23 | 0.3010 (8) | 0.2042 (8) | 0.2072 (8) | 0.0418 (4) | 0.00655 (10) | 0.1008 | 0.94 | 1.23 |
| 0.2040 (6) | 0.2052 (6) | 0.0413 (3) | 0.1012 | |||||||
| 0.84 | 14.18 | 0.3022 (13) | 0.2038 (15) | 0.2045 (17) | 0.0419 (6) | 0.00642 (20) | 0.0868 | 0.72 | 1.21 | |
| 0.2044 (12) | 0.2044 (12) | 0.0408 (5) | 0.0884 | |||||||
| 0.32 | 4.02 | 0.2999 (23) | 0.2014 (18) | 0.2068 (17) | 0.0415 (7) | 0.00652 (35) | 0.0982 | 0.90 | 1.13 | |
| 0.2032 (16) | 0.2032 (13) | 0.0399 (7) | 0.0973 | |||||||
| Blank | 0.19 | 0.2964 (120) | 0.1927 (81) | 0.2177 (110) | 0.0449 (35) | 0.00833 (170) | 0.0388 | |||
| A-π/4 | 0.2026 (72) | 0.1998 (75) | 0.0454 (41) | 0.0386 | ||||||
| 3.75 | 231.4 | 0.3049 (9) | 0.2013 (10) | 0.2033 (10) | 0.0402 (4) | 0.00627 (12) | 0.0517 | 0.17 | 1.04 | |
| 0.2025 (11) | 0.2029 (9) | 0.0396 (3) | 0.0520 | |||||||
| UV-laser ablation. The laser beam is reflected by 45° dichroic mirror (external to the cell) and hits the Al surface at 45° angle X- and Y stages are moving in the same horizontal plane | 0.44 | 5.63 | 0.3007 (27) | 0.2049 (18) | 0.2072 (20) | 0.0391 (7) | 0.00618 (28) | 0.0888 | 0.75 | 0.96 |
| 0.2032 (20) | 0.2065 (17) | 0.0416 (8) | 0.0878 | |||||||
| 0.78 | 12.13 | 0.3010 (32) | 0.2017 (22) | 0.2090 (25) | 0.0419 (13) | 0.00570 (35) | 0.0867 | 0.72 | 1.12 | |
| 0.2030 (23) | 0.2052 (21) | 0.0423 (10) | 0.0867 | |||||||
| 0.15 | 2.57 | 0.2987 (35) | 0.2018 (25) | 0.2081 (29) | 0.0397 (11) | 0.00621 (44) | 0.0797 | 0.61 | 1.04 | |
| 0.2015 (26) | 0.2087 (25) | 0.0417 (11) | 0.0791 | |||||||
| 0.24 | 2.97 | 0.3011 (38) | 0.2017 (29) | 0.2014 (28) | 0.0429 (12) | 0.00611 (51) | 0.0933 | 0.82 | 1.02 | |
| 0.2004 (28) | 0.2029 (25) | 0.0428 (13) | 0.0943 | |||||||
| 0.72 | 10.24 | 0.3020 (24) | 0.2019 (14) | 0.2034 (17) | 0.0408 (6) | 0.00619 (24) | 0.0850 | 0.69 | 0.98 | |
| 0.2023 (18) | 0.2023 (15) | 0.0403 (5) | 0.0854 | |||||||
| A-π | Blank | 0.14 | 0.2913 (140) | 0.1916 (95) | 0.2039 (110) | 0.0420 (48) | 0.00535 (580) | 0.0554 | ||
| 0.1856 (100) | 0.1929 (100) | 0.0387 (50) | 0.0538 | |||||||
| AloS ablated upside down. IR-beam first hits the transparent sapphire substrate and melts Al from the side of the Al-sapphire interface keeping the viewport free of sputtered Al | 1.48 | 20.61 | 0.3003 (19) | 0.2004 (16) | 0.2069 (18) | 0.0402 (7) | 0.00681 (35) | 0.0940 | 0.83 | 1.16 |
| 0.2003 (16) | 0.2056 (16) | 0.0411 (7) | 0.0958 | |||||||
| 0.20 | 3.37 | 0.3038 (50) | 0.1993 (49) | 0.2043 (42) | 0.0385 (22) | 0.00665 (63) | 0.0836 | 0.67 | 1.13 | |
| 0.2006 (47) | 0.2023 (49) | 0.0407 (20) | 0.0777 | |||||||
| 0.84 | 13.50 | 0.3017 (25) | 0.2048 (22) | 0.2062 (23) | 0.0397 (10) | 0.00601 (44) | 0.0875 | 0.73 | 1.17 | |
| 0.2030 (24) | 0.2054 (19) | 0.0402 (13) | 0.0893 | |||||||
| 0.32 | 3.55 | 0.3019 (38) | 0.2016 (31) | 0.2034 (33) | 0.0422 (14) | 0.00555(130) | 0.0985 | 0.90 | 1.00 | |
| 0.2018 (35) | 0.2055 (28) | 0.0409 (13) | 0.1012 | |||||||
| 0.24 | 3.38 | 0.3022 (62) | 0.2019 (48) | 0.2054 (58) | 0.0413 (19) | 0.00567 (83) | 0.0946 | 0.84 | 1.19 | |
| 0.2037 (51) | 0.2050 (53) | 0.0401 (19) | 0.0961 | |||||||
| 0.80 | 10.38 | 0.3047 (16) | 0.2024 (12) | 0.2052 (12) | 0.0440 (5) | 0.00640 (20) | 0.0910 | 0.78 | 1.02 | |
| 0.2036 (13) | 0.2074 (12) | 0.0409 (5) | 0.0912 | |||||||
| P-π/4 | Blank | 0.38 | 0.2997(60) | 0.1979 (50) | 0.2098 (72) | 0.0495 (24) | 0.00677 (68) | 0.0667 | ||
| 0.2035 (52) | 0.2063 (48) | 0.0456 (25) | 0.0685 | |||||||
| PAC ablated by the UV-beam tuned by external 45° mirror. Same as A-π/4 but different collector material: PAC instead of AloS | 8.40 | 98.41 | 0.3030 (6) | 0.2031 (4) | 0.2044 (4) | 0.0409 (4) | 0.00634 (18) | 0.0901 | 0.77 | 0.90 |
| 0.2021 (4) | 0.2039 (4) | 0.0421 (4) | 0.0905 | |||||||
| 2.04 | 26.73 | 0.3013 (9) | 0.2042 (7) | 0.2049 (8) | 0.0411 (3) | 0.00631 (30) | 0.0839 | 0.67 | 0.88 | |
| 0.2020 (7) | 0.2048 (8) | 0.0408 (3) | 0.0848 | |||||||
| 0.86 | 13.84 | 0.3007 (9) | 0.2030 (7) | 0.2038 (7) | 0.0412 (3) | 0.00611 (30) | 0.0760 | 0.55 | 0.88 | |
| 0.2033 (7) | 0.2059 (7) | 0.0417 (3) | 0.0743 | |||||||
| 0.42 | 8.75 | 0.3037 (17) | 0.2028 (13) | 0.2039 (11) | 0.0409 (6) | 0.00638 (55) | 0.0694 | 0.45 | 0.93 | |
| 0.2018 (13) | 0.2029 (11) | 0.0419 (6) | 0.0702 | |||||||
| Atmospheric Kr | 0.3052 | 0.2014 | 0.2022 | 0.0396 | 0.00609 | 0.0415 |
Notes: Numbers in parenthesis are 1σ. Errors for gas concentrations and elemental ratios are 5–7% based on the scatter observed in series of air standards measured prior and after each experiment. 132Xe/84Kr = 0.041 was used to resolve SW from trapped Kr.