Table 2.
Entry | Substrate | Product | Product [mm] | TON | TOF [h−1] |
---|---|---|---|---|---|
1 | 989 | 424 | 17.7 | ||
2 | 87.5 | 37.5 | 1.6 | ||
3 | 330 | 142 | 5.9 | ||
4 | 235 | 101 | 4.2 | ||
5 | 179/15.7[c] | 76.8/11.0[c] | 3.2/0.5[c] | ||
6 | 359/63.6[c] | 154/44.5[c] | 6.4/1.9[c] | ||
7 | 440 | 188 | 7.8 | ||
8[b] | 307 | 65.7 | 2.7 | ||
9 | 412 | 177 | 7.4 | ||
10 | 514 | 220 | 9.2 | ||
11 | 27.5 | 11.8 | 0.5 | ||
12 | 69.9 | 30.0 | 1.3 | ||
13 | 44.3 | 19.0 | 0.8 |
[a] Conditions: alcohol/water [c(SAS)aq=1 mm]=3:7, O2 atmosphere, T=30 °C, λ>400 nm, reaction time: 24 h; values correspond to the concentration in the organic phase; TON=molproduct×molSAS −1; TOF=TON×24 h−1. [b] c(SAS)aq=2 mm was used, t=48 h. [c] Product concentration in water phase.