(a) Scanning electron micrographs of gradient hydrogels (GelMA- MκCA). A significant increase in pore size was observed at the interface and MκCA regions, compared to the GelMA region. Compression testing of gradient hydrogels revealed a gradual decrease in compressive moduli when shifting from GelMA region to MκCA region. (b) The addition of nanosilicates (nSi) increased the overall gradient hydrogel pore size with a significant increase in the interface and MκCA nSi regions compared to the GelMA nSi region. Similarly, mechanical testing revealed a gradual decrease in compressive moduli but the inclusion of nSi increased the overall compressive moduli two-fold. (Statistical Analysis: One-way Anova with Tukey’s post-hoc analysis, * p-value<0.05, ** p-value< 0.01, *** p-value<0.001, ****p-value<0.0001)