Table 3. DFT Relative Energies and Conformational Populations of Riolozatrione (1) and 6-epi-Riolozatrione (2).
conformer | ΔEmPW1B95 | %OPT | ΔGmPW1B95 | %mPW1B95 | ΔEB3PW91 | %OPT | ΔGB3PW91 | %B3PW91 |
---|---|---|---|---|---|---|---|---|
1a | 0.36 | 25.54 | 0.00 | 56.92 | 0.00 | 43.24 | 0.00 | 51.17 |
1b | 1.02 | 8.31 | 1.03 | 10.05 | 0.94 | 8.80 | 0.40 | 25.92 |
1c | 0.00 | 46.49 | 0.62 | 20.10 | 0.05 | 39.94 | 0.63 | 17.61 |
1d | 0.51 | 19.66 | 0.88 | 12.93 | 1.00 | 8.02 | 1.34 | 5.29 |
2a | 0.00 | 69.23 | 0.00 | 86.00 | 0.00 | 61.42 | 0.00 | 56.84 |
2b | 0.84 | 16.88 | 1.17 | 11.06 | 0.94 | 12.78 | 0.57 | 21.75 |
2c | 1.45 | 6.03 | 2.44 | 1.33 | 0.91 | 13.22 | 0.77 | 15.41 |
2d | 1.29 | 7.86 | 1.59 | 5.57 | 0.94 | 12.57 | 1.33 | 5.98 |