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(a) pH-dependent reactivity of Mn(III) porphyrins for halide oxidation and the acid-base equilibria between the trans-dioxoMn(V), oxo–hydroxo Mn(V), and oxo-aqua Mn(V) species. (b) Synthesis of a trans-dioxoMn(V) porphyrin 54. (c) Characterization of 54 via rR and IR spectroscopies. (d) Mn–O bond length vs 1/F1/3(Mn–O). (c) and (d) were adapted from ref (233). Copyright 2007 American Chemical Society.
