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(a) Proposed mechanism for the oxidative rearrangement of pentalenolactone F catalyzed by PntM. (b) Active site structures of PntM with bound pentalenolactone F (PDB: 5L1O). (c) Steric environment of C1 si and re sides of pentalenolactone F and hydroxylation of 1-deoxypentalenic acid by CYP105D7.
