Figure 2.
Assessing the reactivity of a thioester reporter in complex proteomes. (a) Strategy for ex situ (lysate) and in situ (cellular) labeling using thioester 1. (b) Dose-dependent ex situ labeling of cancer cell lysates by thioester 1 (A549, 15 h, 0, 100, 200, 400, 800 μM). (c) Labeling by 1 is competed by acetyl-CoA (1 h pre-incubation with 0, 100, 200, 400, or 800 μM acetyl-CoA, then 400 μM 1 for 15 h). (d) Dose-dependent in situ labeling of cancer cell by thioester 1 (A549, 15 h, 0, 100, 200, 400, 800 μM).