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Time evolution of the spin‐orbit free state populations (thin lines) in the first 500 fs of the excited‐state dynamics of 2NN. The populations of the excited triplet states Tn (n=2–6) have been combined into one. See Figure S5 in the Supporting Information for the individual contributions of all triplet states. Thick lines represent fits based on the first‐order processes given in Equation (1).
