Fig. 3. Photon energy scaling for intraband heating.
(A) The THz photoconductivity ΔσTHz as a function of pump pulse fluence, parametrized by the photoexcited carrier density nexc, for two pump photon energies Eph = 1.0 eV (purple circles) and 2.5 eV (green circles). The solid lines serve as guides to the eye based on saturation curves. These measurements are done at Vg = 0 V, where we measure a DC conductivity of σ0 ≈ 8 e2/h. Using the mobility of ~1000 cm2/Vs, we extract an equilibrium Fermi energy of |EF| ≃ 0.25 eV, corresponding to graphene gated away from the charge neutrality point. The THz photoconductivity saturates for nctexc ≳ 0.05 × 1012/cm2, corresponding to a relatively low-incident fluence < 1 μJ/cm2, as observed earlier (27, 30). The signal (and therefore the hot-carrier density) is larger for the larger photon energy. Thus, larger photon energies are responsible for larger hot-carrier densities. This is a key signature of efficient intraband heating (25). (B) The THz photoconductivity at nexc = 0.2 × 1012/cm2 [vertical dashed line in (A)], as a function of the pump photon energy. The solid circles are experimental data (right vertical axis) and the solid line the result of the theoretical calculation (left vertical axis) for EF = 0.25 eV. Experiment and theory show good qualitative agreement, with a larger absolute value of the THz photoconductivity for larger photon energy. (C) The calculated hot-CM factor HCM, defined in the main text, as a function of the pump photon energy. The HCM-factor increases with photon energy. (D) The electron distributions and the state occupation in the Dirac cone, compare with Fig. 2, before and after photoexcitation with pump photon energy Eph = 2.5 eV (left, green wavy line) and 1.0 eV (right, purple wavy line). The broadening of the electron distribution is larger in the Eph = 2.5 eV case, indicating more intraband heating for larger photon energy.