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. 2018 Aug 1;57(35):11247–11251. doi: 10.1002/anie.201805244

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© 2018 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.

This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.

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Scheme 1 — Mechanistic pathways for water oxidation with the final O−O formation via nucleophilic attack of water to the ruthenium–oxo species (WNA, blue; that is, Ru(phenda)(pic)₂ 10) or via interaction of two metal–oxo moieties (I2M, red; that is, Ru(bda)(pic)₂ 8b,8c).