Table 1.
No. | Rt (min) | Compounds | Molecular Formula | Molecular Weight | Main Mass Fragments | Area% in RR Fruit | Area% in RS Fruit |
---|---|---|---|---|---|---|---|
1 | 3.12 | 3-Furaldehyde | C5H4O2 | 96 | 67, 39 | - | 0.01 ± 0.001 |
2 | 3.17 | Furfural | C5H4O2 | 96 | 67, 39 | 0.67 ± 0.03 | 0.57 ± 0.02 |
3 | 3.34 | 3-Hexen-1-ol | C6H12O | 100 | 83, 67, 41 | - | 0.53 ± 0.01 |
4 | 3.40 | 4-Methyl-octane | C9H20 | 128 | 112, 85, 71, 69, 43 | 0.83 ± 0.04 | 0.17 ± 0.01 |
5 | 3.41 | Ethyl benzene | C8H10 | 106 | 91, 74, 51, 27 | - | 0.20 ± 0.02 |
6 | 3.48 | o-Xylene | C8H10 | 106 | 91, 74, 51 | 0.3 ± 0.003 | - |
7 | 3.48 | p-Xylene | C8H10 | 106 | 91, 74, 51 | - | 0.28 ± 0.02 |
8 | 3.67 | Styrene | C8H8 | 104 | 78, 51, 27 | 1.53 ± 0.05 | 0.04 ± 0.003 |
9 | 4.27 | 5-Methyl-nonane | C10H22 | 142 | 112, 85, 65, 43 | 0.16 ± 0.003 | - |
10 | 4.94 | 2-Ethyl-1-hexanol | C8H18O | 130 | 112, 83, 57, 29 | 0.23 ± 0.01 | - |
11 | 4.99 | d-Limonene | C10H16 | 158 | 137, 121, 93, 68, 41 | 0.22 ± 0.01 | 0.17 ± 0.01 |
12 | 5.02 | Benzyl alcohol | C7H8O | 108 | 79, 51 | - | 0.02 ± 0.002 |
13 | 5.07 | 1,6-Dimethylhepta-1,3,5-triene | C9H14 | 122 | 107, 91, 65, 41 | - | 0.03 ± 0.002 |
14 | 5.16 | 3,7-Dimethyl-1,3,6-octatriene | C10H16 | 136 | 121, 93, 77, 57 | - | 0.05 ± 0.01 |
15 | 5.69 | 4,5-Diethyloctane | C12H26 | 170 | 141, 111, 84, 67, 43 | 0.63 ± 0.02 | 0.46 ± 0.02 |
16 | 5.94 | 1,2,4,5-Tetramethylbenzene | C10H14 | 134 | 119, 91, 65 | - | 0.01 ± 0.001 |
17 | 6.01 | 5,6-Dimethyldecane | C12H26 | 170 | 141, 113, 84, 67, 43 | 0.73 ± 0.02 | 0.18 ± 0.02 |
18 | 6.17 | 4-Ethyldecane | C12H26 | 170 | 140, 113, 85, 43 | 0.18 ± 0.01 | - |
19 | 6.24 | 2,6-Dimethyldecane | C12H26 | 170 | 140, 113, 71, 43 | 0.29 ± 0.01 | - |
20 | 6.68 | Dodecane | C12H26 | 170 | 141, 112, 85, 57, 41 | 0.14 ± 0.01 | - |
21 | 7.05 | 2-Carene | C10H16 | 136 | 121, 93, 77 | - | 0.03 ± 0.003 |
22 | 7.22 | 2,6,10-Trimethyldodecane, | C15H32 | 212 | 183, 155, 127, 85, 57 | - | 0.02 ± 0.002 |
23 | 7.29 | 1,2,3,4-Tetrahydro-1,1,6-trimethylnaphthalene | C13H18 | 174 | 159, 131, 105, 71 | - | 0.07 ± 0.01 |
24 | 7.46 | 3-Methylnonadecane | C20H42 | 283 | 253, 169, 141, 113, 85, 57 | 0.12 ± 0.01 | - |
25 | 7.65 | 2,3-Dihydro-1,1,5,6-tetramethyl-1H-indene | C6H7BClNO3 | 187 | 159, 128, 91, 71 | - | 0.26 ± 0.02 |
26 | 7.66 | Decane | C10H22 | 142 | 99, 71, 43, 27 | 0.03 ± 0.004 | - |
27 | 8.23 | 1,1,5-Trimethyl-1, 2-dihydronaphthalene | C13H16 | 172 | 157, 141, 115, 77 | - | 0.07 ± 0.01 |
28 | 8.28 | Megastigma-4,6(Z),8(Z)-triene | C13H20 | 176 | 161, 133, 105, 77 | - | 0.04 ± 0.004 |
29 | 8.47 | Dichloroacetic acid, tetradecyl ester | C16H30Cl2O2 | 325 | 196, 168, 139, 111, 83, 65, 43 | 0.07 ± 0.006 | - |
30 | 8.47 | 1-Tetradecene | C14H28 | 196 | 168, 140, 111, 83 | - | 0.04 ± 0.003 |
31 | 8.53 | Tetradecane | C14H30 | 198 | 169, 141, 113, 85, 57 | 0.03 ± 0.003 | - |
32 | 8.74 | Alloaromadendrene | C15H24 | 204 | 189, 161, 119, 91, 69 | - | 0.06 ± 0.004 |
33 | 8.99 | 3,8-Dimethyldecane | C12H26 | 170 | 141, 113, 85, 57 | - | 0.08 ± 0.01 |
34 | 9.04 | 9-Methylnonadecane | C20H42 | 282 | 267, 238, 168, 140, 113, 85 | - | 0.03 ± 0.004 |
35 | 9.20 | 2,6-Bis(1,1-dimethylethyl)-2,5-cyclohexadiene-1,4-dione | C14H20O2 | 220 | 177, 135, 91, 67 | - | 0.07 ± 0.01 |
36 | 9.51 | 2,4-Bis(1,1-dimethylethyl)phenol | C14H22O | 206 | 191, 163, 115, 91, 57 | 0.13 ± 0.01 | 0.13 ± 0.02 |
37 | 9.60 | 1-Butyl-2-propylcyclopentane | C12H24 | 168 | 140, 111, 91, 69, 41 | 0.03 ± 0.004 | - |
38 | 9.65 | 4-Ethoxybenzoic acid ethyl ester | C11H14O3 | 194 | 149, 121, 93, 65 | - | 0.09 ± 0.01 |
39 | 9.87 | Dodecanoic acid | C12H24O2 | 200 | 157, 129, 101, 73, 43 | 0.54 ± 0.02 | 2.26 ± 0.09 |
40 | 10.15 | 1-Tricosanol | C23H48O | 340 | 322, 294, 154, 125, 97, 69, 43 | 0.08 ± 0.01 | - |
41 | 10.22 | Hexadecane | C16H34 | 226 | 169, 141, 113, 85, 57 | 0.12 ± 0.02 | - |
42 | 11.26 | 2,6,10,14-Tetramethylpentadecane | C19H40 | 268 | 253, 183, 141, 113, 85, 57 | - | 0.20 ± 0.01 |
43 | 11.33 | Heptadecane | C17H36 | 240 | 169, 141, 113, 85, 57 | 0.21 ± 0.01 | 5.38 ± 0.13 |
44 | 11.49 | 3,7,11-Trimethyl-1,6,10-dodecatrien-3-ol | C15H26O | 222 | 204, 161, 136, 93, 69 | 0.24 ± 0.02 | - |
45 | 11.72 | Hexacosane | C26H54 | 366 | 243, 197, 141, 113, 85, 57 | - | 0.09 ± 0.004 |
46 | 11.83 | 9-Octylheptadecane | C25H52 | 352 | 239, 197, 169, 141, 113, 85, 57 | 0.09 ± 0.01 | - |
47 | 11.86 | Tetradecanoic acid | C14H28O2 | 228 | 185, 157, 129, 97, 73 | 0.44 ± 0.02 | 0.92 ± 0.02 |
48 | 12.08 | Benzyl benzoate | C14H12O2 | 212 | 167, 105, 77, 51 | - | 0.27 ± 0.01 |
49 | 12.23 | 6-Tetradecanesulfonic acid butyl ester | C18H38O3S | 334 | 196, 127, 91, 71, 52 | - | 0.08 ± 0.01 |
50 | 12.28 | 3,3,4-Trimethyl-4-p-tolylcyclopentanol | C15H22O | 218 | 200, 163, 147, 119, 91 | 0.20 ± 0.01 | - |
51 | 12.50 | 2,6,10,14-Tetramethylhexadecane | C20H42 | 282 | 253, 183, 141, 113, 85 | 0.18 ± 0.01 | - |
52 | 13.06 | 2-Methylheptadecane | C18H38 | 254 | 239, 211, 141, 113, 85, 57 | - | 0.11 ± 0.01 |
53 | 13.25 | Cyclohexadecane | C16H32 | 224 | 125, 55 | - | 0.16 ± 0.02 |
54 | 13.40 | 1,2-Benzenedicarboxylic acid bis(2-methylpropyl) ester | C16H22O4 | 278 | 223, 167, 149, 104, 76, 57 | 0.44 ± 0.03 | 0.28 ± 0.01 |
55 | 13.49 | Cyclopentadecane | C15H30 | 210 | 182, 139, 111, 83, 55 | 0.07 ± 0.001 | - |
56 | 13.63 | 2-Methylhexacosane | C27H56 | 380 | 365, 337, 169, 141, 113, 85 | - | 0.10 ± 0.01 |
57 | 13.68 | Hentriacontane | C31H64 | 436 | 169, 141, 113, 85, 57 | - | 0.14 ± 0.01 |
58 | 13.69 | 8-Heptadecene | C17H34 | 238 | 210, 140, 111, 83, 55 | 0.08 ± 0.001 | - |
59 | 14.21 | 2,3-Dimethylnonadecane | C21H44 | 297 | 253, 183, 155, 127, 99, 71 | 0.19 ± 0.01 | - |
60 | 14.53 | Palmitoleic acid | C16H30O2 | 254 | 236, 192, 137, 111, 83 | 0.77 ± 0.02 | - |
61 | 14.57 | Oxacycloheptadecan-2-one | C16H30O2 | 254 | 236, 194, 138, 111, 83 | 0.39 ± 0.01 | - |
62 | 14.87 | n-Hexadecanoic acid a | C16H32O2 | 256 | 213, 185, 157, 129, 83, 60 | 16.06 ± 0.25 | 20.86 ± 0.31 |
63 | 15.64 | 1-Heptacosanol | C27H56O | 396 | 378, 181, 153, 125, 97, 57 | 0.29 ± 0.02 | - |
64 | 16.06 | 3,7,11,15-Tetramethylhexadeca-1,3,6,10,14-pentaene | C20H32 | 272 | 229, 191, 119, 93, 69 | 0.65 ± 0.01 | - |
65 | 16.07 | 3,7,11-Trimethyl-2,6,10-dodecatrien-1-ol | C15H26O | 222 | 191, 161, 137, 93, 69 | - | 0.70 ± 0.01 |
66 | 16.12 | Trispiro[4.2.4.2.4.2.]heneicosane | C21H44 | 296 | 288, 231, 192, 163, 135, 97 | 0.29 ± 0.01 | - |
67 | 16.47 | N-[4-bromo-n-butyl]-2-piperidinone | C9H16BrNO | 234 | 205, 154, 97, 43 | - | 0.10 ± 0.01 |
68 | 16.73 | 2,2-Dimethyl-5-(3-methyloxiranyl)-cyclohexanone | C11H20O2 | 196 | 182, 153, 123, 95, 69, 41 | 0.11 ± 0.008 | - |
69 | 16.74 | 7-Bromomethylpentadec-7-ene | C16H31Br | 302 | 223, 153, 125, 97, 69 | - | 0.15 ± 0.01 |
70 | 17.03 | 1-Nonadecene | C19H38 | 266 | 266, 210, 168, 126, 97 | 0.31 ± 0.01 | 0.10 ± 0.01 |
71 | 17.04 | 8-Hexadecene | C16H32 | 224 | 196, 153, 125, 97, 69 | - | 0.60 ± 0.02 |
72 | 17.21 | Estra-1,3,5(10)-trien-17β-ol | C18H24O | 256 | 185, 157, 129, 97, 73 | - | 0.11 ± 0.01 |
73 | 17.23 | Nonadecyl pentafluoropropionate | C22H39F5O2 | 430 | 313, 266, 153, 125, 97, 57 | 0.03 ± 0.001 | - |
74 | 17.36 | Heneicosane | C21H44 | 296 | 197, 169, 141, 113, 85 | 0.63 ± 0.02 | 0.51 ± 0.02 |
75 | 17.64 | 6-Octen-1-ol, 3,7-dimethyl acetate | C12H22O2 | 198 | 156, 123, 103, 81 | 2.33 ± 0.15 | - |
76 | 17.94 | Trifluoroacetic acid pentadecyl ester | C18H31F3O2 | 336 | 306, 255, 182, 140, 111, 83 | - | 0.42 ± 0.02 |
77 | 18.09 | 9,12-Octadecadienoic acid a | C18H32O2 | 280 | 236, 150, 123, 95, 67 | 2.92 ± 0.09 | 0.59 ± 0.01 |
78 | 18.21 | 9,12,15-Octadecatrien-1-ol | C18H32O | 264 | 236, 208, 108, 79 | 6.66 ± 0.14 | - |
79 | 18.40 | 9,12,15-Octadecatrienoic acid a | C18H30O2 | 278 | 222, 163, 135, 108, 79 | - | 9.06 ± 0.17 |
80 | 18.66 | 4-(4-Ethylcyclohexyl)-1-pentylcyclohexene | C19H34 | 262 | 220, 191, 164, 123, 81 | 0.42 ± 0.01 | - |
81 | 18.66 | Methyl 6,9,12-hexadecatrienoate | C17H28O2 | 264 | 194, 175, 135, 107, 79 | - | 0.69 ± 0.02 |
82 | 18.80 | 9-Octadecenoic acid a | C18H34O2 | 282 | 264, 222, 165, 137, 111, 83 | 0.43 ± 0.01 | 0.14 ± 0.01 |
83 | 18.83 | 1-Eicosene | C20H40 | 280 | 252, 182, 153, 125, 97 | 0.53 ± 0.02 | 0.10 ± 0.01 |
84 | 18.84 | tert-Hexadecanethiol | C16H34S | 258 | 224, 165, 111, 57 | - | 0.74 ± 0.01 |
85 | 18.97 | Bacchotricuneatin C | C20H22O5 | 342 | 245, 191, 145, 112, 71 | - | 0.14 ± 0.01 |
86 | 19.01 | E-8-Methyl-7-dodecen-1-ol acetate | C15H28O2 | 240 | 197, 165, 126, 97, 69 | 0.08 ± 0.003 | - |
87 | 19.01 | 3-Methylheptadecane | C18H38 | 254 | 225, 169, 141, 113, 85, 57 | - | 0.12 ± 0.01 |
88 | 19.03 | 1-Chloro-octadecane | C18H37Cl | 288 | 175, 147, 113, 85, 57 | - | 0.50 ± 0.01 |
89 | 19.15 | 2-Dodecen-1-yl(-)succinic anhydride | C16H26O3 | 266 | 237, 299, 181, 149, 123, 97, 69, 41 | 0.07 ± 0.001 | 0.10 ± 0.01 |
90 | 19.21 | 1-(1,5-Dimethylhexyl)-4-(4-methylpentyl)cyclohexane | C20H40 | 280 | 191, 166, 123, 97, 69 | 0.05 ± 0.001 | 0.27 ± 0.01 |
91 | 19.68 | 9-Tricosene | C23H46 | 322 | 294, 167, 139, 111, 83 | 0.95 ± 0.03 | 0.89 ± 0.02 |
92 | 19.83 | 13-Tetradecen-1-ol acetate | C16H30O2 | 254 | 194, 167, 139, 111, 83 | 0.13 ± 0.01 | - |
93 | 20.55 | 1-Tricosene | C23H46 | 322 | 196, 169, 139, 111, 83, 57 | 0.05 ± 0.001 | - |
94 | 20.92 | 1,7,11-Trimethyl-4-(1-methylethyl)cyclotetradecane | C20H40 | 280 | 236, 204, 165, 125, 97 | 0.10 ± 0.01 | 0.12 ± 0.01 |
95 | 21.03 | 1-Docosene | C23H46 | 308 | 223, 181, 139, 97, 57 | 0.33 ± 0.01 | 0.18 ± 0.01 |
96 | 21.34 | Eicosyl pentafluoropropionate | C23H41F5O2 | 444 | 426, 280, 182, 153, 125, 97 | 0.09 ± 0.005 | 0.16 ± 0.01 |
97 | 21.66 | Eicosane | C20H42 | 282 | 197, 169, 141, 113, 85 | 1.10 ± 0.04 | 2.28 ± 0.10 |
98 | 21.91 | Docosane | C22H46 | 310 | 197, 169, 141, 113, 85 | 0.04 ± 0.003 | 0.37 ± 0.01 |
99 | 22.05 | Nonadecane | C19H40 | 268 | 197, 169, 141, 113, 85 | 0.68 ± 0.01 | - |
100 | 22.06 | Octatriacontyl trifluoroacetate | C40H77F3O2 | 646 | 181, 139, 97, 57 | - | 0.46 ± 0.01 |
101 | 22.61 | Behenyl chloride | C22H45Cl | 344 | 189, 169, 141, 113, 85 | 0.44 ± 0.01 | 0.05 ± 0.004 |
102 | 22.72 | 11,13-Dimethyl-12-tetradecen-1-ol acetate | C18H34O2 | 282 | 267, 208, 151, 123, 95, 69 | 0.10 ± 0.02 | 0.69 ± 0.02 |
103 | 22.72 | 15-Isobutyl-(13αH)-isocopalane | C24H44 | 332 | 276, 219, 191, 151, 123, 95 | - | 0.41 ± 0.01 |
104 | 24.21 | Cyclotetracosane | C24H48 | 336 | 308, 167, 139, 111, 83 | 0.41 ± 0.01 | 0.49 ± 0.01 |
105 | 24.32 | 2,2'-Methylenebis[6-(1,1-dimethylethyl)-4-methyl]phenol | C23H32O2 | 340 | 284, 177, 149, 121, 91 | 2.78 ± 0.09 | 2.51 ± 0.07 |
106 | 24.59 | Hexadecyloxirane | C18H36O | 268 | 250, 211, 166, 138, 111, 82 | 0.71 ± 0.03 | - |
107 | 25.48 | Dotriacontyl pentafluoropropionate | C35H65F5O2 | 612 | 594, 448, 181, 139, 97, 57 | 0.08 ± 0.002 | 0.13 ± 0.01 |
108 | 26.38 | Tetratriacontane | C34H70 | 478 | 253, 225, 197, 169, 141, 113, 85 | - | 0.39 ± 0.02 |
109 | 26.66 | 12-Pentacosene | C25H50 | 350 | 350, 181, 153, 125, 97, 69 | 0.20 ± 0.01 | - |
110 | 27.32 | Bis(2-ethylhexyl)phthalate | C24H38O4 | 390 | 279, 180, 149, 104, 57 | 1.60 ± 0.06 | - |
111 | 27.95 | Eicosyl trifluoroacetate | C22H41F3O2 | 394 | 376, 325, 280, 153, 125, 97 | 0.06 ± 0.002 | - |
112 | 28.50 | Heptacosyl trifluoroacetate | C29H55F3O2 | 492 | 474, 423, 378, 181, 139, 97 | 0.09 ± 0.01 | - |
113 | 28.58 | Hexacosane | C26H54 | 366 | 169, 141, 113, 85, 57 | 1.11 ± 0.05 | 1.20 ± 0.06 |
114 | 29.31 | 2-Dodecen-1-yl(-)succinic anhydride | C16H26O3 | 266 | 209, 166, 137, 97, 69 | 1.65 ± 0.06 | 0.08 ± 0.002 |
115 | 29.53 | Tricosane | C23H48 | 324 | 197, 169, 141, 113, 85 | 0.13 ± 0.01 | 0.53 ± 0.02 |
116 | 29.88 | Pentacosane | C25H52 | 352 | 211, 169, 141, 113, 85, 57 | - | 1.56 ± 0.05 |
117 | 29.89 | 2,6,10,14,18-Pentamethyleicosane | C25H52 | 352 | 253, 183, 141, 113, 85 | 1.15 ± 0.04 | - |
118 | 30.64 | 2,6,10,14-Tetramethyl-7-(3-methylpent-4-enylidene)pentadecane | C25H48 | 348 | 264, 207, 167, 125, 97 | 0.56 ± 0.02 | - |
119 | 30.67 | 14-Nonacosane | C29H60 | 408 | 378, 181, 153, 125, 97 | 0.25 ± 0.01 | 0.10 ± 0.03 |
120 | 30.87 | Octadecane | C18H38 | 254 | 169, 141, 113, 85, 57 | 8.16 ± 0.14 | 5.70 ± 0.09 |
121 | 31.05 | 1-Hexacosene | C26H52 | 364 | 209 ,181, 153, 125, 97 | 0.46 ± 0.01 | 0.54 ± 0.02 |
122 | 31.59 | 1-Bromo-11-iodoundecane | C11H22BrI | 362 | 281, 233, 177, 135, 97 | 0.31 ± 0.01 | 0.27 ± 0.01 |
123 | 31.62 | 1-Methyl-4-(1-methylethyl)-3-[1-methyl-1-(4-methylpentyl)-5-methylheptyl]cyclohexene | C25H48 | 348 | 248, 193, 123, 69 | 0.24 ± 0.01 | - |
124 | 32.46 | 13-Methyl-Z-14-nonacosene | C30H60 | 420 | 405, 209, 181, 153, 125, 97 | 0.78 ± 0.02 | - |
125 | 32.98 | (5α,14β)-Cholestane | C27H48 | 372 | 259, 218, 176, 149, 109 | 2.11 ± 0.03 | 1.66 ± 0.09 |
126 | 33.10 | Tetracosane | C24H50 | 338 | 169, 141, 113, 85, 57 | 3.24 ± 0.05 | 1.00 ± 0.07 |
127 | 33.67 | Cholestane | C27H48 | 372 | 262, 217, 149, 109, 81 | 5.24 ± 0.09 | 3.93 ± 0.10 |
128 | 34.33 | (5α,13α)-d-Homoandrostane | C20H34 | 274 | 259, 217, 177, 149, 95, 55 | 1.25 ± 0.04 | 1.39 ± 0.06 |
129 | 35.31 | Nonacosane | C29H60 | 408 | 197, 169, 141, 113, 85 | 6.44 ± 0.21 | 5.07 ± 0.19 |
130 | 35.94 | Stigmastane | C29H52 | 400 | 290, 217, 189, 149, 109 | 4.44 ± 0.18 | 3.27 ± 0.14 |
131 | 37.45 | 1-Iodo-octadecane | C18H37I | 380 | 253, 183, 141, 99, 57 | 2.16 ± 0.08 | 0.67 ± 0.03 |
132 | 37.46 | Triacontane | C30H62 | 422 | 197, 169, 141, 113, 85, 57 | - | 2.88 ± 0.11 |
133 | 37.80 | 28-Nor-17α(H)-hopane | C29H50 | 398 | 383, 355, 218, 191, 137, 109 | 2.44 ± 0.09 | - |
134 | 43.31 | β-Sitosterol | C29H50O | 414 | 381, 329, 255, 213, 145, 81 | 4.60 ± 0.17 | 2.36 ± 0.09 |
135 | 43.70 | (3β,24Z)-Stigmasta-5,24(28)-dien-3-ol | C29H48O | 412 | 379, 314, 281, 229, 202 | - | 2.04 ± 0.10 |
a Compounds were confirmed by the reference standards. RR: R. roxburghii; RS: R. sterilis.