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Concept of photocatalytic proton reduction catalysis by 1⋅Fe4(Zn‐L)6. Top left: Molecular structure of cage Fe4(Zn‐L)6. Top right: Molecular structure of [FeFe]hydrogenase mimic 1. Bottom: Concept of photoinduced electron transfer from the supramolecular cage to the encapsulated catalyst, followed by the reduction of protons to molecular hydrogen.
