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a) Overview of CrI3 monolayer and MP‐intercalated bilayer CrI3. b) The switching of net magnetization (marked by red arrows) upon FE switching (marked by blue arrows). c) Energy profile of FE switching pathway for MP‐intercalated bilayer CrI3 (M = Ti and V). d) Monte Carlo simulation of temperature dependence of magnetization for pristine CrI3 monolayer and the layer binding with VP.
