Table A1.
Calculated electronic energies, zero-point(ZP)-corrected electronic energies, enthalpies and Gibbs free energies at 25 °C in the gas phase for HStLi and HSt2Li, their dimers, and intermediates and products of their reaction with styrene.
Structure designation | System a | State b | Sym. c | Electronic energy | ZP-Corrected El. energy | Enthalpy at 25 °C | Free energy at 25 °C |
---|---|---|---|---|---|---|---|
Hartree | Hartree | Hartree | Hartree | ||||
Styrene | Cs | −309.509791 | −309.375108 | −309.367380 | −309.406880 | ||
1-a, 17-a | (HStLi)2 | Ci | −635.361832 | −635.066685 | −635.047732 | −635.112274 | |
1-b | (HStLi)2 | C2 | −635.362034 | −635.066958 | −635.048066 | −635.111985 | |
1-c | (HStLi)2 | C2 | −635.357316 | −635.062952 | −635.043667 | −635.108167 | |
1-d | (HStLi)2 | C1 | −635.357150 | −635.062696 | −635.043457 | −635.108156 | |
1-e | (HStLi)2 | C1 | −635.340616 | −635.045969 | −635.026702 | −635.093660 | |
1-f | (HStLi)2 | C1 | −635.340376 | −635.045695 | −635.026400 | −635.094205 | |
2-a, 18-d | HStLi | C1 | −317.636426 | −317.490146 | −317.480837 | −317.522499 | |
2-b | HStLi | C1 | −317.636468 | −317.490098 | −317.480959 | −317.522120 | |
2-c, 18-a | HStLi | C1 | −317.639063 | −317.492539 | −317.483239 | −317.524976 | |
4-a | St/HStLi(2-a) | trans. st. | C1 | −627.164750 | −626.881101 | −626.864941 | −626.924697 |
6-a | ditto | prec. com. | C1 | −627.177240 | −626.894714 | −626.877210 | −626.939206 |
6-c, 10-a | ditto | prod. | C1 | −627.203797 | −626.917733 | −626.901515 | −626.960375 |
4-b, | St/HStLi(2-a) | trans. st. | C1 | −627.165509 | −626.882034 | −626.866082 | −626.924258 |
10-b | ditto | prod. | C1 | −627.203635 | −626.917030 | −626.901097 | −626.959118 |
4-c | St/HStLi(2-b) | trans. st. | C1 | −627.163789 | −626.880182 | −626.864094 | −626.923495 |
4-d | St/HStLi(2-c) | trans. st. | C1 | −627.171213 | −626.888516 | −626.872055 | −626.931624 |
5-a | ditto | prec. com. | C1 | −627.182144 | −626.899522 | −626.882012 | −626.943264 |
5-c, 10-c | ditto | prod. | C1 | −627.209000 | −626.922552 | −626.906625 | −626.963788 |
4-e | St/HStLi(2-c) | trans. st. | C1 | −627.170339 | −626.887312 | −627.870970 | −626.930497 |
10-d | ditto | prod. | C1 | −627.208225 | −626.921535 | −626.905769 | −626.962507 |
9-a | (HSt2Li)2 | C1 | −1,254.473434 | −1,253.899128 | −1,253.866430 | −1,253.962071 | |
9-b | (HSt2Li)2 | C2 | −1,254.475478 | −1,253.901031 | −1,253.868215 | −1,253.964187 | |
9-c | (HSt2Li)2 | C1 | −1,254.472061 | −1,253.898082 | −1,253.865322 | −1,253.962687 | |
9-d | (HSt2Li)2 | C2 | −1,254.475433 | −1,253.900563 | −1,253.868171 | −1,253.961955 | |
9-e | (HSt2Li)2 | Ci | −1,254.465490 | −1,253.890015 | −1,253.857141 | −1,253.955849 | |
9-f | (HSt2Li)2 | C2 | −1,254.465572 | −1,253.891320 | −1,253.858378 | −1,253.958174 | |
10-e | HSt2Li | C1 | −627.190521 | −626.904064 | −626.887908 | −626.947895 | |
10-f | HSt2Li | C1 | −627.190042 | −626.903752 | −626.887554 | −626.947817 | |
10-g | HSt2Li | C1 | −627.188224 | −626.902301 | −626.885951 | −626.946715 | |
10-h | HSt2Li | C1 | −627.189002 | −626.902981 | −626.886712 | −626.946723 | |
11-a | St/HSt2Li(10-c) | trans. st. | C1 | −936.719842 | −936.296363 | −936.273546 | −936.345734 |
12-a | ditto | init. com. | C1 | −936.733277 | −936.310954 | −936.286633 | −936.363099 |
12-b | ditto | sub-trans. st. | C1 | −936.730098 | −936.307908 | −936.284255 | −936.360239 |
12-c | ditto | prec. com. | C1 | −936.738992 | −936.316726 | −936.292352 | −936.369237 |
12-e | ditto | prod. | C1 | −936.754519 | −936.328104 | −936.305247 | −936.378605 |
11-b | St/HSt2Li(10-c) | trans. st. | C1 | −936.714658 | −936.291484 | −936.268399 | −936.343249 |
11-c | St/HSt2Li(10-d) | trans. st. | C1 | −936.716195 | −936.291972 | −936.269438 | −936.340815 |
11-d | St/HSt2Li(10-d) | trans. st. | C1 | −936.712791 | −936.288519 | −936.265940 | −936.338335 |
11-e | St/HSt2Li(10-e) | trans. st. | C1 | −936.722598 | −936.300214 | −936.276740 | −936.354197 |
11-f | St/HSt2Li(10-e) | trans. st. | C1 | −936.721523 | −936.298977 | −936.275484 | −936.353934 |
11-g | St/HSt2Li(10-f) | trans. st. | C1 | −936.722896 | −936.300627 | −936.277131 | −936.354853 |
13-a | ditto | prec. com. | C1 | −936.734032 | −936.311594 | −936.287128 | −936.366417 |
13-c | ditto | prod. | C1 | −936.761364 | −936.335489 | −936.312428 | −936.387432 |
11-h | St/HSt2Li(10-f) | trans. st. | C1 | −936.722064 | −936.299676 | −936.276150 | −936.354137 |
11-i | St/HSt2Li(10-g) | trans. st. | C1 | −936.715325 | −936.292112 | −936.268776 | −936.347402 |
11-j | St/HSt2Li(10-g) | trans. st. | C1 | −936.714844 | −936.291764 | −936.268515 | −936.346813 |
11-k | St/HSt2Li(10-h) | trans. st. | C1 | −936.716557 | −936.293320 | −936.270052 | −936.348016 |
11-m | St/HSt2Li(10-h) | trans. st. | C1 | −936.716907 | −936.293762 | −936.270585 | −936.347825 |
a ‘ditto’ here means that not only the structure of HStmLi but also the arrangement of styrene vs. HStmLi are the same as those of the upper column; b trans. st.: transition state, prec. com.: precursor complex, prod.: product, init. com.: initial complex, sub-trans. st.: sub-transition state; c sym.: symmetry.