Table 1.
Entry | [M] | Base | 2 (equiv) | Time (h) | Yield of 3a (%) 1 |
---|---|---|---|---|---|
1 | FeCl2 | CsF | 1.5 | 24 | 29 |
2 | CoCl2 | CsF | 1.5 | 24 | 21 |
3 | NiCl2 | CsF | 1.5 | 24 | 90 |
4 | NiBr2 | CsF | 1.5 | 24 | 68 |
5 | Ni(cod)2 | CsF | 1.5 | 24 | 16 |
6 | PdCl2 | CsF | 1.5 | 24 | 4 |
7 | NiCl2 | Cs2CO3 | 1.5 | 24 | 48 |
8 | NiCl2 | KF | 1.5 | 24 | 0 |
9 | NiCl2 | CsF | 1.2 | 24 | 94 (90) |
10 | NiCl2 | CsF | 1.0 | 24 | 58 |
11 | NiCl2 | CsF | 1.2 | 18 | 91 |
12 | NiCl2 | CsF | 1.2 | 12 | 87 |
13 | NiCl2 | CsF | 1.2 | 6 | 76 |
1 Determined by GC analysis of the crude mixture using n-dodecane as an internal standard. An isolated yield is given in parentheses.