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. 2019 Dec 31;11(8):2243–2259. doi: 10.1039/c9sc05432d

Table 6. First oxidation potentials (EO1, V vs. Fc+/0) of group 8 metal carbene complexes supported by the TPFPP macrocycle.

Complex E O1 a (V) Ref. b
Fe-mono(carbene) complexes
[Fe(TPFPP)(Ad)] (1a) 0.01 TW
[Fe(TPFPP)(CPh2)] 0.35 17g
Ru-mono(carbene) complexes
[Ru(TPFPP)(Ad)] (2a) 0.18 TW
[Ru(TPFPP)(CPh2)] 0.46 17g
[Ru(TPFPP)(C(Ph)CO2Me)(MeOH)] 0.65 17g
Os-bis(carbene) complexes
[Os(TPFPP)(Ad)2] (3b) 0.04 c TW
[Os(TPFPP)(CPh2)2] 0.30 TW

a E 1/2 values of reversible oxidation processes.

bTW = this work.

cQuasi-reversible.