Table 2.
Analysis laboratory | Analysis method | S solution 233Pa massic activity (Bq g−1) | S solution molality of 233Pa (pmol g−1) |
NIST | LTAC* | 26,320 ± 170 | 0.1470 ± 0.0010 |
NIST | HPGe γ spectrometry | 26,120 ± 570 | 0.1459 ± 0.0032 |
NRC | LTAC* | 26,190 ± 370 | 0.1463 ± 0.0021 |
NRC | Coincidence counting | 26,340 ± 450 | 0.1471 ± 0.0025 |
NRC | TDCR | 26,310 ± 220 | 0.1469 ± 0.0012 |
NRC | CNET 1 | 26,040 ± 230 | 0.1454 ± 0.0013 |
NRC | CNET 2 | 26,130 ± 250 | 0.1459 ± 0.0014 |
NPL | Coincidence counting* | 26,340 ± 180 | 0.1471 ± 0.0010 |
Analysis laboratory | Analysis method | M solution 231Pa massic activity (Bq g−1) | RM solution molality of 231Pa (pmol g−1) |
NIST | α Spectrometry* | 2096 ± 68 | 27.6 ± 1.0 |
NIST | CNET Corrected | 2154 ± 67 | 28.41 ± 0.73 |
NIST | CNET | 2175 ± 67 | 28.7 ± 1.0 |
NRC | CNET* | 2193 ± 66 | 28.92 ± 0.98 |
NRC | TDCR | 2266±41 | 29.88 ± 0.72 |
Molality of 233Pa was converted from massic activity using the evaluated 233Pa half-life [12] of (26.98 ± 0.2) days (k = 1). The molality of 231Pa in the RM solution was calculated from the M solution massic activity using the dilution factor of 187.279 ± 0.047 (k = 2) and the evaluated 231Pa half-life [11] of (32 670 ± 260) a (k = 1). All values are decay corrected to a reference time of 27 June 2017 22:50 UTC. Uncertainties are expanded uncertainties (U=k uc) with a coverage factor (k) of 2. NIST massic activity values are from [13] for 233Pa and [15] for 231Pa. All massic activity values for NRC are from [14] and the cited 233Pa activity value from NPL is from Keightley (personal communication, 7 February 2018). CNET 1 and 2 refer to analyses performed on liquid scintillation counters from different manufacturers
Primary or highest confidence activity measurements, as designated by the analysis laboratories