Table 2.
Pesticides that were analyzed in this study and their chemical properties.
| Pesticide type | Application method on bananaa | Substance group | Active ingredient | Mol. weightb | LogKOWb | LogKOAc | Solubility (mg/L)b | Henry’s Constant (Pa.m3/mol)d | Vapor pressure (25°) (mPa)d | Volatilityd |
|---|---|---|---|---|---|---|---|---|---|---|
| Insecticides | Treated bag | Organophosphate | Chlorpyrifos | 350.58 | 4.96 | 8.40 | 0.39 | 0.478 | 1.43 | Moderate volatile |
| Thiadiazine | Buprofezine | 305.44 | 4.93 | 8.97 | 0.90 | 2.8 x 10−02 | 0.04 | Non-volatile | ||
| Not reported | Organophosphate to be used on banana | Diazinonf | 304.34 | 3.69 | 8.89 | 60 | 6.09 x 10−02 | 11.97 | Non-volatile | |
| Nematicides | Manual | Carbamate | Carbofuran | 221.25 | 2.32 | 8.11 | 351 | 5.0 x 10−05 | 0.08 | Non-volatile |
| dispenser | Organophosphate | Cadusafos | 270.38 | 3.90 | 8.18 | 245 | 0.13 | 119.60 | Moderatelyvolatile | |
| Ethoprophosg | 242.33 | 3.59 | 8.77 | 750 | 1.35 x 10−02 | 78.00 | Non-volatile | |||
| Fenamiphos | 303.35 | 3.23 | 9.72 | 329 | 9.90 x 10−05 | 0.12 | Non-volatile | |||
| Terbufosh | 288.41 | 2.77 | 7.49 | 5.07 | 2.70 | 34.60 | Moderately volatile | |||
| Fungicides | Aerial spraying | Anilinopyrimidine | Pyrimethanil | 199.25 | 2.84 | 8.67 | 121 | 3.60 x 10−03 | 1.10 | Non-volatile |
| Chloronitrile | Chlorothalonili | 265.90 | 2.94 | 8.11 | 0.81 | 2.50 x 10−02 | 0.07 | Non-volatile | ||
| Morpholine | Fenpropimorphj | 303.49 | 4.50j | 8.93 | 4.32 | 2.74 x 10−04 | 3.90 | Non-volatile | ||
| Spiroxamine | 297.48 | 2.89 | 10.87 | 405 | 3.80 x 10−03 | 3.50 | Non-volatile | |||
| Strobilurin | Azoxystrobin | 403.39 | 2.50 | 14.03 | 6.00 | 7.40 x 10−09 | 1.10 x 10−07 | Non-volatile | ||
| Triazole | Bitertanol | 337.42 | 4.10 | 12.17 | 3.80 | 2.60 x 10−07 | 1.36 x 10−06 | Non-volatile | ||
| Difenoconazole | 406.26 | 4.40 | 11.93 | 15.0 | 9.00 x 10−07 | 3.33 x 10−05 | Non-volatile | |||
| Epoxiconazole | 329.75 | 3.30 | 9.11 | 7.1 | 4.71 x 10−04 | 1.00 x 10−02 | Non-volatile | |||
| Propiconazole | 342.22 | 3.72 | 9.24 | 100 | 9.20 x 10−05 | 0.05 | Non-volatile | |||
| Tebuconazole | 307.82 | 3.70 | 10.19 | 36 | 1.00 x 10−05 | 1.30 x 10−03 | Non-volatile |
Reported to be used on banana by Bravo et al. (2013), the following pesticides were also reported but were not analyzed: bifenthrin, mancozeb, tridemorph, pyraclostrobin, trifloxystrobin, diquat, paraquat, glufosinate, glyphosate.
Data on chemical properties are from PubChem https://pubchem.ncbi.nlm.nih.gov, solubility in water at 20 °C, pH 7 (mg/L).
Log KOA (octanol air partition coefficient) is calculated from the log KOW (octanol water partition coefficient) using the ideal gas constant and Henry’s Constant value (Meylan and Howard, 2005).
Data on chemical properties are from IUPAC Pesticides Properties Database (PPDB) https://sitem.herts.ac.uk/aeru/ppdb/en/; According to Gibbs et al. (2017), Henry’s Constant values > 10−8 and logKOA values 7–13 indicate that the compound is ideal for passive sampling with PUF; volatility interpretation according to Henry’s Constant.
Reported to be used together with bifenthrin in bags to protect banana fruit (Ruepert, personal communication).
Not reported to be used on banana.
Also reported to be used on pine-apple.
The metabolite terbufos sulfone was also analyzed.
Was not quantified for Passive Air Sampling (PAS).
Data on chemical properties are from EPA https://www3.epa.gov/pesticides/chem_search/reg_actions/registration/fs_PC-121402_01-Mar-06.pdf.