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Activation strain analysis diagrams for the a, b, c) SN2@C reactions and d, e, f) SN2@Si ambident reactions computed at ZORA‐OLYP/TZ2P. The color of the line indicates the side of the ambident nucleophile reacting with the substrate (black: C, blue: N, red: O, and yellow: S) and the dot (•) indicates the position of the transition state/complex.
