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. 2020 May 12;11:2363. doi: 10.1038/s41467-020-16098-8

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© The Author(s) 2020

Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

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Fig. 1 — a Asymmetry induction in catalytic metal-carbene C(sp²)-H functionalization. b Chirality in transient carbene intermediate. c This work describes the transient axial-chirality-controlled asymmetric C(sp²)–H functionalization. The pink crescent = chiral ligand (L = large group, S = small group). M = metal catalyst. Rh₂L₄* = chiral dirhodium complex.