TABLE 3.
Regression equation, limit of detection (LOD), limit of quantitation (LOQ), intra‐ and inter‐day precision, repeatability, stability, recovery and matrix effect of 50 compounds
| Name | Regression equation | r | Linear range (ng/mL) | LOD (ng/mL) | LOQ (ng/mL) | Precision | Repeatability | Stability | Recovery | Matrix effect | ||
|---|---|---|---|---|---|---|---|---|---|---|---|---|
| Intra‐day (RSD%; n = 6) | Inter‐day (RSD%; n = 3) | (RSD %; n = 6) | (RSD%; n = 6) | Mean | RSD% | |||||||
| Chlorogenic acid | y = 845x + 4.77e5 | 0.9999 | 0.604–755000 | 0.195 | 0.585 | 1.78 | 1.79 | 1.55 | 3.33 | 99.70 | 0.23 | 1.01 |
| Neochlorogenic acid | y = 115x + 1.13e5 | 0.9992 | 3.01–376000 | 0.388 | 1.163 | 1.83 | 1.71 | 0.88 | 1.61 | 96.70 | 3.97 | 1.00 |
| Cryptochlorogenic acid | y = 878x + 6.7e3 | 0.9993 | 0.316–79000 | 0.090 | 0.271 | 4.04 | 4.31 | 2.42 | 2.47 | 100.66 | 1.62 | 1.04 |
| 3,5‐O‐Dicaffeoylquinic acid | y = 1.02e3 x + 1.41e5 | 0.9996 | 77.6–388000 | 14.483 | 43.449 | 2.63 | 2.79 | 0.72 | 1.62 | 98.70 | 2.65 | 0.98 |
| 3,4‐O‐Dicaffeoylquinic acid | y = 602x + 1.45e5 | 0.9995 | 7.63–38200 | 2.094 | 6.282 | 3.95 | 4.39 | 3.14 | 4.94 | 100.67 | 3.65 | 1.02 |
| 4,5‐O‐Dicaffeoylquinic acid | y = 483x + 2.1e4 | 0.9998 | 45–28100 | 7.918 | 23.755 | 3.27 | 3.64 | 1.16 | 1.62 | 98.40 | 2.12 | 1.01 |
| 1,3‐O‐Dicaffeoylquinic acid | y = 5.78e3 x + 5.62e4 | 0.9996 | 42–2630 | 6.971 | 20.913 | 3.44 | 3.28 | 2.82 | 3.16 | 100.92 | 3.43 | 1.04 |
| Caffeic acid | y = 2.49e3 x + 1.69e5 | 0.9998 | 5.76–7200 | 1.169 | 3.506 | 2.86 | 3.17 | 3.29 | 4.83 | 101.17 | 2.05 | 1.03 |
| Quinic acid | y = 1.19e3 x + 3.05e5 | 0.9996 | 19.6–245000 | 5.131 | 15.392 | 2.73 | 2.38 | 1.69 | 4.18 | 100.20 | 2.48 | 1.05 |
| Protocatechuic acid | y = 6.13e3 x + 1.95e5 | 0.9994 | 7.68–960 | 0.780 | 2.341 | 2.50 | 2.30 | 4.09 | 3.85 | 99.50 | 2.82 | 0.96 |
| Ferulic acid | y = 121x + 3.68e3 | 0.999 | 11.2–1400 | 2.814 | 8.441 | 4.21 | 3.96 | 3.69 | 3.58 | 102.08 | 4.88 | 0.99 |
| 4,5‐O‐Dicaffeoylquinic acid methyl ester | y = 9.67e3 x – 4.3e4 | 0.9996 | 5.6–700 | 1.319 | 3.958 | 3.79 | 4.10 | 1.78 | 1.78 | 98.20 | 3.48 | 0.97 |
| Rutin | y = 2.5e3 x + 3.14e5 | 0.9998 | 0.979–12200 | 0.036 | 0.108 | 2.91 | 3.21 | 3.31 | 3.46 | 95.90 | 3.99 | 1.03 |
| Hyperoside | y = 4.32e3 x + 1.77e5 | 0.9995 | 0.265–3313 | 0.058 | 0.174 | 1.69 | 1.55 | 3.21 | 3.22 | 100.32 | 3.82 | 1.03 |
| Luteoloside | y = 1.07e3 x + 1.34e5 | 1 | 0.664–41500 | 0.056 | 0.169 | 1.03 | 0.92 | 4.64 | 3.78 | 99.16 | 2.95 | 1.01 |
| Luteolin | y = 100x + 2.47e3 | 0.9995 | 124–15600 | 10.150 | 30.450 | 2.28 | 2.22 | 1.34 | 4.09 | 100.29 | 4.35 | 1.00 |
| Rhoifolin | y = 1.08e4 x + 572 | 0.9999 | 1.3–162 | 0.280 | 0.840 | 2.53 | 2.75 | 5.20 | 4.64 | 99.82 | 3.14 | 0.97 |
| Diosmetin | y = 1.15e4 x – 9.93e3 | 0.9993 | 1.72–214 | 0.146 | 0.438 | 1.09 | 0.78 | 4.63 | 2.31 | 100.93 | 2.95 | 0.99 |
| Apigenin | y = 2.17e4 x – 9.13e4 | 0.9995 | 25.4–318 | 4.188 | 12.563 | 3.54 | 3.83 | 3.39 | 3.47 | 103.09 | 3.98 | 0.98 |
| Kaempferol | y = 191x + 250 | 0.9997 | 2.02–101 | 0.565 | 1.695 | 4.28 | 4.68 | 3.59 | 3.32 | 101.27 | 3.01 | 0.95 |
| Astragalin | y = 2.17e4 x + 8.73e4 | 0.9999 | 0.0353–883 | 0.005 | 0.015 | 3.51 | 3.92 | 3.09 | 3.51 | 100.17 | 3.57 | 0.97 |
| Lonicerin | y = 1.11e3 x + 4.25e3 | 0.9994 | 22.4–14000 | 0.024 | 0.073 | 3.45 | 3.85 | 2.95 | 2.74 | 100.74 | 2.80 | 1.01 |
| Kaempferol‐3‐O‐rutinoside | y = 3.13e3 x + 9.11e4 | 0.9999 | 0.632–7900 | 0.039 | 0.117 | 2.31 | 2.44 | 3.79 | 3.36 | 99.82 | 3.18 | 0.98 |
| Isoquercitrin | y = 4.33e3 x + 1.4e5 | 0.9996 | 2.65–3310 | 0.195 | 0.584 | 1.68 | 1.54 | 4.97 | 2.91 | 99.68 | 2.12 | 1.02 |
| Sweroside | y = 34.9x + 1.56e3 | 0.9996 | 0.841–52600 | 0.231 | 0.692 | 3.54 | 3.68 | 3.97 | 4.99 | 101.78 | 2.92 | 1.00 |
| Secologanic acid | y = 609x + 3.48e4 | 0.9999 | 1.45–182000 | 0.072 | 0.217 | 3.02 | 3.37 | 4.87 | 2.19 | 99.32 | 4.05 | 1.03 |
| Loganin | y = 3.95x + 1.72e3 | 0.999 | 14.1–35200 | 4.179 | 12.536 | 2.26 | 2.43 | 1.83 | 1.18 | 103.36 | 3.89 | 0.99 |
| Secoxyloganin | y = 638x + 1.32e5 | 0.999 | 0.189–47400 | 0.052 | 0.157 | 4.19 | 4.67 | 2.47 | 4.68 | 98.42 | 3.14 | 1.02 |
| Loganin acid | y = 1.11e3 x – 1.98e5 | 0.9993 | 441.2–22100 | 139.266 | 417.797 | 2.95 | 2.54 | 4.60 | 4.55 | 100.32 | 2.60 | 1.03 |
| Morroniside | y = 10.4x + 8.21e3 | 0.999 | 41.1–514000 | 7.867 | 23.600 | 2.11 | 1.83 | 4.32 | 3.03 | 101.75 | 4.18 | 0.98 |
| Macranthoidin A | y = 193x + 9.76e3 | 0.9997 | 18.1–22600 | 2.989 | 8.967 | 2.72 | 1.94 | 2.43 | 2.70 | 103.97 | 3.66 | 1.01 |
| Dipsacoside B | y = 8.94x + 336 | 0.9999 | 3.34–20900 | 0.745 | 2.236 | 2.25 | 2.37 | 3.18 | 3.84 | 99.81 | 0.92 | 1.01 |
| Akebia saponin D | y = 6.02x + 8.06e3 | 0.9996 | 16.6–207000 | 1.539 | 4.618 | 3.10 | 1.65 | 1.46 | 1.05 | 102.90 | 4.10 | 0.94 |
| l‐Alanine | y = 1.43e3 x + 1.78e4 | 0.9997 | 8.47–10600 | 2.228 | 6.684 | 3.07 | 2.60 | 4.50 | 3.43 | 101.09 | 4.66 | 1.03 |
| l‐Serine | y = 351x + 5.93e4 | 0.9997 | 9.16–11500 | 1.342 | 4.027 | 2.71 | 2.54 | 3.31 | 3.40 | 99.84 | 1.96 | 1.02 |
| l‐Proline | y = 1.77e3 x + 3.04e4 | 0.9996 | 0.381–23800 | 0.093 | 0.279 | 2.75 | 2.86 | 2.84 | 1.13 | 102.36 | 2.19 | 1.01 |
| l‐Valine | y = 6.36e3 x + 2.17e5 | 0.9995 | 2.51–1570 | 0.215 | 0.644 | 2.96 | 3.19 | 1.49 | 3.33 | 98.52 | 3.85 | 1.04 |
| l‐Threonine | y = 1.75e3 x – 9.1e4 | 0.9996 | 111–13900 | 22.325 | 66.975 | 2.83 | 1.46 | 3.20 | 2.83 | 96.47 | 4.28 | 0.97 |
| l‐Isoleucine | y = 5.15e3 x + 1.92e5 | 0.9998 | 2.88–3600 | 0.422 | 1.265 | 0.67 | 0.63 | 1.27 | 2.54 | 99.49 | 2.45 | 1.00 |
| l‐Leucine | y = 9.64e3 x + 4.72e5 | 0.9997 | 3.38–4230 | 0.711 | 2.134 | 1.21 | 1.28 | 4.23 | 3.05 | 103.97 | 2.36 | 1.01 |
| l‐Aspartic acid | y = 660x + 2.38e4 | 0.9991 | 4.6–57500 | 0.835 | 2.506 | 1.49 | 1.66 | 4.18 | 4.27 | 99.27 | 2.96 | 0.96 |
| l‐Glutamate | y = 1.64e3 x – 2.82e5 | 0.9998 | 474–29600 | 136.177 | 408.530 | 0.69 | 0.74 | 1.71 | 1.53 | 96.93 | 3.96 | 1.04 |
| l‐Lysine | y = 2.32e3 x – 2.01e5 | 0.9993 | 147–12600 | 36.781 | 110.342 | 0.58 | 0.65 | 2.15 | 2.20 | 95.67 | 3.73 | 0.99 |
| l‐Histidine | y = 7.11e3 x + 1.65e5 | 0.9999 | 59.1–7390 | 7.656 | 22.968 | 1.67 | 1.45 | 3.55 | 3.62 | 104.62 | 4.79 | 1.05 |
| l‐Phenylalanine | y = 1.7e4 x + 2.55e5 | 0.9997 | 25.6–3200 | 0.550 | 1.650 | 1.78 | 1.28 | 3.16 | 2.36 | 97.56 | 3.06 | 1.03 |
| l‐Arginine | y = 6.54e3 x + 1.21e5 | 0.9996 | 0.241–1510 | 0.043 | 0.128 | 1.25 | 1.19 | 4.54 | 4.50 | 100.17 | 1.98 | 1.00 |
| Cytidine | y = 4.72e4 x – 1.94e4 | 0.9995 | 1.84–230 | 0.496 | 1.488 | 3.39 | 3.20 | 4.69 | 3.99 | 94.20 | 3.90 | 1.01 |
| Uridine | y = 861x + 7.0e3 | 0.9997 | 40.4–5050 | 7.124 | 21.372 | 3.20 | 3.53 | 4.19 | 3.26 | 100.95 | 2.55 | 1.01 |
| Adenosine | y = 5.28e4 x + 3.05e5 | 0.9994 | 6.31–789 | 0.945 | 2.834 | 1.45 | 1.41 | 1.89 | 3.29 | 97.76 | 3.70 | 0.98 |
| Inosine | y = 7.98e3 x + 2.12e4 | 0.9991 | 8.78–220 | 1.847 | 5.542 | 1.73 | 1.87 | 3.95 | 3.93 | 101.52 | 4.10 | 0.95 |