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Relative difference between the approximate estimates Kd′ (eq 21, eq 13 of de Jong et al.18) and the box-size-independent estimates Kd (eq 1) for the dissociation constant as shown in Figure 6 (discs) as functions of the inverse box volume 1/V. This difference is proportional to 1/V and to the contribution of unbound states to the second osmotic virial coefficient, Bij (eq 41, lines).
