(A) Crystal structure of human DPP3 active site (PDB accession code 3FVY). The location of residues involved in zinc metal binding (H450, H455, E508), the catalytic glutamate (E451), and a non-catalytic tyrosine 417 (Y417) identified by SuTEx are highlighted. (B) Lead SuTEx fragments (JWB142) and negative control probe (JWB131) identified from a gel-based chemical proteomic screen against recombinant DPP3 proteomes (Supplementary Figure 7). (C) JWB142 but not JWB131 blocked catalytic activity of purified DPP3 in a concentration-dependent manner as measured by substrate assay: JWB142, IC50 = 17 μM, 95% confidence intervals: 11-27 μM. JWB142 showed >10-fold increase in inhibitory activity compared with the SuFEx counterpart: SuFEx-3, IC50 = 246 μM, 95% confidence intervals: 117-519 μM. Data are shown as mean ± s.e.m.; n = 3 biologically independent experiments. (D) DPP3 Y417 site is liganded (~50% blockade) by JWB142 but not JWB131 fragment as judged by quantitative chemical proteomic analysis of recombinant human DPP3-HEK293T soluble cell proteome. All data shown are representative of n = 2 biologically independent experiments.