Table 1.
Entry | Catalyst | Temperature (°C) | Conversion (%) | Yield (%) |
---|---|---|---|---|
1 | Blank | 150 | 0 | 0 |
2 | Fe-C900-PCC | 150 | 0 | 0 |
3 | Fe-C900-PCC | 200 | 0 | 0 |
4 | Fe-N900-PCC | 150 | 0 | 0 |
5 | Fe-N900-PCC | 200 | 8 | 7 |
6 | Fe-P900-PCC | 150 | 93 | 92 |
7a | Fe-P900-PCC | 150 | 99 | 98 |
8 | Fe@Fe-C900-PCC | 150 | 0 | 0 |
9 | Fe@Fe-N900-PCC | 150 | 0 | 0 |
10 | P900-PCC-polymer | 150 | 0 | 0 |
11 | Fe-P900-PCC-polymer | 150 | 0 | 0 |
Reaction conditions: 1 mmol quinoline, 100 mg catalyst, 2 mL heptane, 4 MPa H2, and 12 h. The conversion and yield are determined by GC using dodecane as internal standard.
aReaction time is prolonged to 18 h.