Table 1. Energies (kcal mol–1) and Vibrational Harmonic Frequencies (cm–1) of the Stationary Points Along with the Reaction N2O + C2H2 → Oxadiazole.
| frequencies
(cm–1) |
||||||||||||||||
|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|
| species | method | 1 | 2 | 3 | 4 | 5 | 6 | 7 | 8 | 9 | 10 | 11 | 12 | 13 | 14 | 15 |
| N2O + C2H2 (0; 0; 0) | PESa | 582 | 582 | 1291 | 2272 | 572 | 572 | 729 | 729 | 2004 | 3403 | 3498 | ||||
| AVDZb | 584 | 584 | 1295 | 2276 | 552 | 552 | 730 | 730 | 2001 | 3401 | 3493 | |||||
| AVTZc | 600 | 600 | 1301 | 2284 | 616 | 616 | 752 | 752 | 2005 | 3408 | 3501 | |||||
| oxadiazole (−44.54; −44.49; −42.26) | PESa | 584 | 611 | 686 | 781 | 833 | 942 | 967 | 1085 | 1131 | 1147 | 1356 | 1427 | 1547 | 3280 | 3303 |
| AVDZb | 608 | 615 | 679 | 765 | 797 | 938 | 966 | 1091 | 1132 | 1142 | 1356 | 1423 | 1543 | 3279 | 3302 | |
| AVTZc | 595 | 632 | 680 | 733 | 781 | 942 | 972 | 1093 | 1135 | 1143 | 1360 | 1429 | 1548 | 3283 | 3306 | |
| TS (25.00; 25.05; 27.14) | PESa | 585i | 267 | 283 | 486 | 587 | 632 | 704 | 711 | 731 | 820 | 1285 | 1807 | 1890 | 3372 | 3437 |
| AVDZb | 593i | 281 | 298 | 482 | 566 | 593 | 705 | 706 | 730 | 809 | 1289 | 1815 | 1898 | 3367 | 3436 | |
| AVTZc | 606i | 285 | 305 | 495 | 559 | 619 | 717 | 718 | 761 | 824 | 1265 | 1819 | 1912 | 3372 | 3443 | |
This work, fitted PIP-NN PES.
This work, CCSD(T)-F12a/AVDZ.
This work, CCSD(T)-F12a/AVTZ.