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. 2020 Oct 6;252:117176. doi: 10.1016/j.carbpol.2020.117176

Table 2.

Stabilization of wetting, foam and O/W emulsion films using various types of nonionic polymeric surfactants.

Surfactant Type Research Methodology Major Findings References
Inutec®SP1 Microinterferometric technique of Scheludko–Exerowa was used to measure the stability of foam films at a constant concentration of Inutec®SP1 (2 × 10−5 mol dm-3) and at several NaCl concentrations (1 × 10-4 to 2 mol dm-3). The film thickness was significantly decreased with increasing NaCl concentration, which indicated the stability of the foam film. At 1 × 10−2 mol dm-3 NaCl, the film thickness remained constant at approximately 16 nm. Exerowa et al. (2006)
Inutec®SP1 The microinterferometric method for investigation of thin liquid films described in the monograph of Exerowa-Kruglyakov against a constant concentration of Inutec®SP1 (2 × 10−5 mol dm-3) and at quite a few NaCl concentrations. The O/W emulsion film thickness was approximately 11 nm. The film thickness could be decreased at critical NaCl concentration 5 × 10−2 mol dm-3. Exerowa et al. (2007)
Inutec®SP1, Block and Triblock copolymeric surfactant The microinterferometric thin liquid pressure balance experimental technique was used to calculate the stability of O/W emulsion films against varying NaCl concentrations Emulsions using Inutec®SP1 should be more stable than those using Pluronics ABA copolymers, in particular at high electrolyte concentrations. Exerowa, Gotchev, Gotchev et al. (2009b)
HMI-A, HMI-B, HMI-C, Inutec®SP1 The microinterferometric technique of Scheludko–Exerowa was used to identify the stability of O/W emulsion films at a constant concentration of surfactants (2 × 10−5 mol dm-3) and multiple concentrations of NaCl. HMI-A, HMI-B, and HMI-C were prepared by changing the DS. Thus, one would expect the loop size to decrease as follows: HMI-A > INUTEC®SP1 >HMI-B >HMI-C. The film thickness was markedly decreased with increasing NaCl concentration at a certain level (5 × 10−2 mol dm−3). In all cases, these NBFs are very stable and have a constant thickness up to the highest possible measured capillary pressure of 45 kPa. With the polymeric surfactant possessing the highest DS, the transition to an NBF of thickness 7 nm occurs even at a low capillary pressure of 36 Pa. With a reduction in DS, the loop size increases, and the transition to an NBF of 7 nm occurs at a higher capillary pressure of 0.5 kPa Exerowa, Gotchev et al. (2009c)
Inutec®SP1 The microinterferometric technique of Scheludko–Exerowa was designed to find the stability of O/W emulsion films against different types of electrolytes (Na2SO4 NaCl and Mg2SO4). The film thickness significantly decreased and produced NBFs in all types of electrolyte at a specific capillary pressure, with no observed influence of electrolyte types on the equivalent film thickness, the formation of NBF and disjoining pressure-equivalent film thickness isotherms. Gotchev et al. (2007)
Inutec®SP1 The microinterferometric technique of Scheludko–Exerowa was used to measure the stability of wetting films produced on a hydrophilic silica surface. The stability was evaluated against different Inutec®SP1 concentrations in the presence or absence of Na2SO4 and NaCl. The equilibrium film thickness varied with increasing electrolyte and polymeric surfactant concentrations. The reduction pattern in the equilibrium film thickness can be observed at 10−1 mol dm−3 NaCl, 10−6 mol dm−3 Inutec®SP1 and 10−2 or 1 mol dm−3 Na2SO4. Nedyalkov et al. (2007)
Inutec®SP1, HMI-B, EFKA-4550 The microinterferometric technique of Scheludko–Exerowa was used to measure the stability of wetting films against different types of polymeric surfactants at varying DSs. The wetting films were stable at (Øw ≤25°) for Inutec®SP1 and (Øw ≤20°) for HMI-B. The general trend of change of h with CEFKA is similar to that obtained for Inutec®SP1 and HMI-B. Nedyalkov et al. (2010)
Inutec®SP1 The microinterferometric method for investigating the wetting and O/W emulsion films described in the monograph of Exerowa-Kruglyakov both in aqueous solution and in the presence of different electrolytes (NaCl, Na2SO4, and MgSO4) concentrations have been studied. Emulsion and wetting films could be stabilized using HMI surfactants in the presence of all different types of electrolytes at varying concentrations. Exerowa, Platikanov et al. (2009d)
Inutec®SP1, 0.5HMI, 2HMI 3HMI. The thin liquid film–pressure balance technique has been used to measure the stability of foam and O/W emulsion films against different types of polymeric surfactants that are synthesized by altering the DS. Thus, one would expect the inulin loop size to decrease as follows: 0.5HMI > Inutec®SP1 > 2HMI > 3HMI. NBFs have been found in all types of inulin-based surfactants and had the same thickness of approximately 7 nm. Foam films are unstable at 8 kPa for 2HMI and 150 Pa for 3HMI, whereas for 0.5HMI and Inutec®SP1, the foam films are stable at 100 kPa. Due to the formation of NBFs, the O/W emulsion films are more stable, up to 45 kPa in all HMI synthesized derivatives. Gotchev et al., 2011.

O/W = oil-in-water, NBF = Newton black film, HMI-A, HMI-B, HMI-C and 1HMI, 2HMI, 3HMI = Different types of inulin derivatives with different DSs. DS = degree of substitution.