Table 2.
| Material | τc [μs] | α0 [m−1] | dn/dT × 10−6 [K−1] | ΔT(0, t=3 s) [K] | ΔΦTL [mrad] | ΔΦ10 MHz/10 W – ΔΦ0 [mrad] |
|---|---|---|---|---|---|---|
| N-BK7 | 690 | 0.12 | 1.2 [23] | 0.82 | 18 | 334 ± 36 |
| CaF2 | 100 | 0.08 | −11.5 [24] | 0.07 | −16 | 172 ±29 |
| MgF2 | 54 | 4.00 | 1.0 [24] | 1.83 | 33 | 40 ± 25 |
| BaF2 | 61 | 0.03 | −16.2 [24] | 0.03 | −5 | −7 ± 18 |
Thermo-optic coefficients (dn/dT) for CaF2, Baf2, and MgF2 were taken from Feldman et al. [24] at 293 K and λ = 1.15 μm.
dn/dT for borosilicate glass (N-BK7) was taken from Frey et al. [23] at 295 K and λ = 1 μm.
Temperatures at the beam center after 3 s exposure to 1 μJ, 300 fs laser pulses at 10 MHz repetition rate ΔT(0, t = 3 s) were determined from heat transfer simulations (Fig. 4).
ΔΦTL the predicted thermal phase shift from our simulations, ΔΦ0 is the measured average nonlinear phase shift from 10 kHz z-scans, and ΔΦ10 WHz/10 W is the measured phase shift during 10 MHz/10 W z-scans.
The last column shows the difference between ΔΦ10 MHz/10 W and ΔΦ0, which should be similar to ΔΦTL if linear-absorption-induced thermal lensing is the primary mechanism contributing to the increase in measured phase shift during high-repetition-rate/high-average-power z-scans.