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Intermolecular Rh-catalyzed synthesis of dehydropiperidines. (A) Select substrates from the aziridine and diazoester scopes of the [3+3] ring expansion of bicyclic aziridines. (B) Computed reaction profile for the process involving aziridine 11b and dirhodium-bound carbene 19a-Rh2. (C) Chirality transfer experiment using enantiopure aziridine (S,R)-11g.
