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Left: Proposed structures of S=2 TauD‐J based on DFT studies; [2] middle: selected examples of S=1 and S=2 oxoiron(IV) cores in TBP and Oh geometries; right: A pseudotetrahedral S=2 oxoiron(IV) complex 2 reported in this work; in the inset is shown the DFT calculated structure of 2 in the S=2 state.
