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. 2021 Feb 10;60(13):6932–6937. doi: 10.1002/anie.202014374

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© 2021 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH

This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc-nd/4.0/ License, which permits use and distribution in any medium, provided the original work is properly cited, the use is non‐commercial and no modifications or adaptations are made.

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Results of spatially resolved a) EDX measurements at each MA of ML2 illustrating the continuous composition gradients; b) XRD measurements of ML2 and a selected diffraction pattern of the MA Pd₄₆Pt_19.2Ru_17.9Ir_16.8Ag_0.1; c) visualisation of APT results from a CSS thin film sputtered on a tip‐array ^[20] to confirm the single‐phase CSS state. The overall composition of this sample as determined by APT is Pd_47.1Pt_18.9Ru_17.8Ir_15.9Ag_0.3.