TABLE 2.
Class | Metabolite | Serum vs. ACD | Serum vs. citrate | Serum vs. EDTA | Serum vs. fluoride | Serum vs. heparin | ||||||||||||||||||||
---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|
Mean diff | SEM | %CV | p-value a | Effect size b | Mean diff | SEM | %CV | p-value a | Effect size b | Mean diff | SEM | %CV | p-value a | Effect size b | Mean diff | SEM | %CV | p-value a | Effect size b | Mean diff | SEM | %CV | p-value a | Effect size b | ||
Amino Acids and their metabolites | 2-Aminobutyrate | 2.1 | 0.6 | 87.1 | 0.624 | 0.22 | 1.7 | 0.6 | 100.7 | 0.687 | 0.18 | 0.5 | 0.4 | 241.3 | 0.935 | 0.06 | −0.3 | 3.9 | −3,356.8 | 0.959 | −0.04 | 0.2 | 0.6 | 980.6 | 0.935 | 0.06 |
2-Hydroxybutyrate | 11.0 | 1.3 | 32.7 | 0.027 | 1.52 | 6.4 | 0.6 | 27.9 | 0.126 | 0.80 | 2.6 | 0.3 | 36.8 | 0.781 | 0.33 | 0.4 | 2.2 | 1,527.1 | 0.959 | 0.05 | 1.8 | 0.8 | 121.0 | 0.858 | 0.20 | |
2-Hydroxyisovalerate | 2.1 | 0.5 | 66.1 | 0.167 | 0.91 | 1.0 | 0.3 | 93.7 | 0.332 | 0.36 | 0.5 | 0.2 | 90.1 | 0.781 | 0.17 | 0.3 | 1.6 | 1,460.7 | 0.632 | 0.11 | 0.5 | 0.1 | 86.5 | 0.858 | 0.16 | |
2-Oxoisocaproate | 1.7 | 0.3 | 45.2 | 0.031 | 1.51 | 0.8 | 0.2 | 50.4 | 0.373 | 0.63 | 0.5 | 0.1 | 50.2 | 0.831 | 0.39 | 0.2 | 0.8 | 1,255.0 | 0.784 | 0.14 | 0.2 | 0.1 | 136.1 | 0.887 | 0.14 | |
3-Hydroxyisobutyrate | 3.8 | 0.4 | 26.7 | 0.027 | 1.82 | 2.4 | 0.2 | 22.1 | 0.086 | 1.09 | 0.5 | 0.3 | 178.9 | 0.879 | 0.22 | 1.4 | 0.7 | 129.2 | 0.513 | 0.66 | 0.5 | 0.2 | 106.9 | 0.858 | 0.24 | |
3-Methyl-2-oxobutanoate | 5.1 | 0.6 | 33.6 | 0.019 | 1.83 | 2.4 | 0.3 | 35.7 | 0.186 | 0.74 | 1.2 | 0.3 | 65.3 | 0.781 | 0.35 | 0.6 | 2.1 | 953.6 | 0.887 | 0.19 | 0.4 | 0.4 | 251.0 | 0.858 | 0.13 | |
Alanine | 96.2 | 6.8 | 19.9 | 0.023 | 1.78 | 83.9 | 4.6 | 15.5 | 0.039 | 1.47 | 39.8 | 4.3 | 30.9 | 0.696 | 0.65 | 79.6 | 29.2 | 103.7 | 0.141 | 1.38 | 39.8 | 4.6 | 32.8 | 0.858 | 0.63 | |
Arginine | 18.2 | 2.6 | 39.6 | 0.018 | 1.96 | 17.7 | 2.2 | 34.6 | 0.021 | 1.75 | 13.9 | 3.8 | 77.6 | 0.148 | 1.65 | 13.8 | 6.3 | 129.7 | 0.141 | 1.33 | 13.2 | 3.5 | 75.7 | 0.341 | 1.12 | |
Asparagine | 14.1 | 1.3 | 27.0 | 0.018 | 1.81 | 10.7 | 1.8 | 47.0 | 0.047 | 1.39 | 3.9 | 0.9 | 65.9 | 0.781 | 0.46 | 10.5 | 3.6 | 95.8 | 0.191 | 1.23 | 4.1 | 1.4 | 96.8 | 0.858 | 0.47 | |
Betaine | 6.4 | 1.5 | 64.3 | 0.370 | 0.37 | 8.9 | 1.3 | 41.6 | 0.332 | 0.55 | 1.6 | 0.6 | 117.2 | 0.879 | 0.09 | 8.6 | 6.6 | 219.2 | 0.434 | 0.53 | 1.9 | 0.9 | 134.7 | 0.887 | 0.11 | |
Glutamate | 3.3 | 2.6 | 219.7 | 0.562 | 0.41 | 20.7 | 2.3 | 31.9 | 0.005 | 2.83 | 5.8 | 3.2 | 156.3 | 0.781 | 0.67 | 10.2 | 4.6 | 127.0 | 0.141 | 1.13 | 14.1 | 1.5 | 30.8 | 0.174 | 1.49 | |
Glutamine | 101.1 | 9.9 | 27.8 | 0.027 | 1.66 | 80.7 | 5.9 | 20.7 | 0.047 | 1.37 | 34.4 | 9.3 | 76.8 | 0.669 | 0.55 | 79.9 | 31.7 | 112.1 | 0.141 | 1.30 | 24.1 | 9.6 | 112.0 | 0.858 | 0.36 | |
Glycine | 66.9 | 5.7 | 23.9 | 0.031 | 1.35 | 58.6 | 3.4 | 16.6 | 0.047 | 1.13 | 8.4 | 1.9 | 63.3 | 0.869 | 0.15 | 50.3 | 34.2 | 192.1 | 0.141 | 0.97 | 26.4 | 3.4 | 36.8 | 0.812 | 0.49 | |
Histidine | 12.6 | 2.2 | 49.1 | 0.031 | 1.59 | 6.9 | 2.1 | 85.7 | 0.263 | 0.86 | −0.9 | 0.9 | -284.3 | 0.879 | −0.12 | 14.4 | 5.8 | 112.8 | 0.141 | 1.55 | 5.0 | 1.9 | 108.3 | 0.858 | 0.52 | |
Isoleucine | 12.6 | 1.1 | 25.1 | 0.096 | 1.18 | 8.9 | 1.1 | 34.6 | 0.223 | 0.82 | 3.1 | 0.6 | 55.3 | 0.869 | 0.28 | 3.3 | 7.5 | 652.2 | 0.631 | 0.29 | 3.6 | 0.9 | 73.0 | 0.858 | 0.31 | |
Leucine | 21.7 | 1.9 | 24.4 | 0.050 | 1.28 | 20.4 | 2.3 | 31.2 | 0.076 | 1.20 | 8.8 | 1.0 | 30.5 | 0.781 | 0.47 | 9.3 | 12.1 | 368.1 | 0.498 | 0.49 | 5.4 | 1.9 | 99.1 | 0.858 | 0.29 | |
Lysine | 29.3 | 2.5 | 24.1 | 0.096 | 1.09 | 24.1 | 2.3 | 27.0 | 0.186 | 0.88 | 5.1 | 2.1 | 115.2 | 0.879 | 0.19 | 21.8 | 12.4 | 160.4 | 0.390 | 0.78 | 9.7 | 1.9 | 54.9 | 0.858 | 0.34 | |
Methionine | 7.6 | 0.5 | 20.0 | 0.007 | 2.82 | 4.9 | 0.4 | 23.9 | 0.027 | 1.67 | 1.5 | 0.7 | 126.1 | 0.869 | 0.46 | 1.7 | 1.9 | 319.1 | 0.365 | 0.52 | 1.3 | 0.7 | 147.1 | 0.858 | 0.39 | |
N,N-Dimethylglycine | 0.6 | 0.1 | 37.8 | 0.096 | 1.01 | 0.4 | 0.1 | 44.0 | 0.332 | 0.67 | 0.2 | 0.1 | 152.0 | 0.879 | 0.24 | 0.3 | 0.4 | 386.3 | 0.579 | 0.44 | 0.1 | 0.0 | 87.4 | 0.858 | 0.15 | |
Ornithine | 28.0 | 2.9 | 29.5 | 0.007 | 2.42 | 24.5 | 2.8 | 32.3 | 0.012 | 1.98 | 12.8 | 1.7 | 37.6 | 0.461 | 0.91 | 15.8 | 8.4 | 150.9 | 0.166 | 1.18 | 13.7 | 1.9 | 40.0 | 0.692 | 0.93 | |
Phenylalanine | 12.1 | 0.4 | 10.1 | 0.018 | 2.02 | 10.3 | 0.7 | 20.4 | 0.031 | 1.76 | 6.8 | 0.4 | 18.3 | 0.416 | 1.06 | 7.9 | 3.7 | 132.7 | 0.166 | 1.18 | 7.8 | 1.1 | 38.6 | 0.174 | 1.17 | |
Proline | 41.5 | 4.5 | 30.6 | 0.142 | 1.01 | 33.9 | 5.8 | 48.3 | 0.126 | 0.82 | 11.4 | 3.1 | 77.5 | 0.869 | 0.25 | 23.0 | 27.5 | 337.8 | 0.390 | 0.53 | 13.0 | 2.9 | 62.9 | 0.858 | 0.29 | |
Serine | 36.1 | 3.5 | 27.2 | 0.040 | 1.54 | 37.2 | 3.0 | 22.6 | 0.031 | 1.58 | 19.5 | 3.3 | 47.6 | 0.593 | 0.77 | 32.0 | 14.2 | 125.4 | 0.166 | 1.27 | 20.4 | 2.2 | 29.9 | 0.812 | 0.78 | |
Taurine | 13.2 | 4.6 | 97.9 | 0.083 | 0.94 | 91.0 | 5.5 | 17.1 | 0.002 | 6.07 | 87.4 | 5.7 | 18.3 | 0.004 | 6.08 | 80.6 | 4.5 | 15.9 | 0.004 | 5.14 | 79.2 | 4.9 | 17.5 | 0.008 | 6.93 | |
Threonine | 24.7 | 2.7 | 31.1 | 0.031 | 1.02 | 20.4 | 2.8 | 38.5 | 0.076 | 0.85 | 4.1 | 2.9 | 201.2 | 0.928 | 0.15 | 13.4 | 10.2 | 215.6 | 0.291 | 0.51 | 6.9 | 2.0 | 80.6 | 0.858 | 0.26 | |
Tryptophan | −0.6 | 0.3 | −164.7 | 0.672 | −0.48 | 1.4 | 0.4 | 87.1 | 0.086 | 1.16 | 0.7 | 0.4 | 168.9 | 0.696 | 0.74 | 1.2 | 0.6 | 141.9 | 0.166 | 1.22 | 0.8 | 0.4 | 166.7 | 0.812 | 0.74 | |
Tyrosine | 11.6 | 0.7 | 17.6 | 0.040 | 1.37 | 9.4 | 0.9 | 27.8 | 0.061 | 1.10 | 3.3 | 0.5 | 44.6 | 0.869 | 0.36 | 5.2 | 6.0 | 327.1 | 0.390 | 0.57 | 4.2 | 1.0 | 65.6 | 0.812 | 0.44 | |
Valine | 51.4 | 3.7 | 20.1 | 0.018 | 1.64 | 38.6 | 3.1 | 22.3 | 0.086 | 1.18 | 12.8 | 2.5 | 55.3 | 0.869 | 0.36 | 16.6 | 20.4 | 348.6 | 0.513 | 0.46 | 15.4 | 3.6 | 66.0 | 0.858 | 0.42 | |
Ketone bodies | 3-Hydroxybutyrate | 16.0 | 5.0 | 88.3 | 0.329 | 0.36 | 14.1 | 5.2 | 103.1 | 0.332 | 0.30 | −8.9 | 8.5 | −269.0 | 0.935 | −0.03 | −9.0 | 13.8 | −431.7 | 0.959 | −0.05 | 2.4 | 4.1 | 476.1 | 0.979 | 0.01 |
Acetoacetate | 2.3 | 1.8 | 224.6 | 0.672 | 0.24 | −28.1 | 0.7 | −7.3 | 0.027 | −1.78 | 8.2 | 5.9 | −202.2 | 0.869 | −0.22 | −8.7 | 6.7 | −217.6 | 0.700 | −0.25 | −2.3 | 0.8 | −102.4 | 0.858 | −0.15 | |
Acetone | −13.4 | 1.4 | −29.2 | 0.115 | −1.24 | −94.5 | 5.9 | −17.6 | 0.002 | −3.71 | −0.2 | 0.6 | −997.6 | 0.935 | −0.03 | 1.8 | 3.9 | 598.3 | 0.631 | 0.14 | 1.3 | 0.6 | 126.3 | 0.858 | 0.08 | |
Lipid metabolism | Carnitine | 0.7 | 1.0 | 426.3 | 1.000 | 0.13 | 6.2 | 0.9 | 41.1 | 0.031 | 1.57 | −0.3 | 1.5 | −1,298.8 | 0.999 | −0.04 | 4.7 | 2.3 | 136.6 | 0.166 | 1.09 | 0.9 | 0.6 | 209.4 | 0.858 | 0.19 |
O-Acetylcarnitine | 2.4 | 0.1 | 17.4 | 0.027 | 1.63 | 2.0 | 0.3 | 34.5 | 0.086 | 1.35 | 0.2 | 0.5 | 650.1 | 0.879 | 0.17 | 0.8 | 0.7 | 243.8 | 0.513 | 0.58 | 0.2 | 0.5 | 573.5 | 0.979 | 0.15 | |
Others | Choline | 1.5 | 0.2 | 32.1 | 0.050 | 1.20 | 1.9 | 0.2 | 28.9 | 0.021 | 1.60 | −1.5 | 2.0 | −389.6 | 0.935 | −0.26 | 0.5 | 0.9 | 511.1 | 0.632 | 0.38 | 0.8 | 0.1 | 43.2 | 0.812 | 0.61 |
Dimethyl sulfone | 1.7 | 0.3 | 42.7 | 0.167 | 0.87 | 1.2 | 0.1 | 33.2 | 0.332 | 0.60 | 0.0 | 0.3 | 3,146.6 | 0.879 | −0.07 | 0.3 | 1.0 | 825.3 | 0.819 | 0.14 | 0.4 | 0.2 | 132.6 | 0.858 | 0.18 | |
Methanol | −40.2 | 2.1 | −14.8 | 0.010 | −2.06 | −1.4 | 1.1 | −220.0 | 0.751 | −0.20 | 0.1 | 0.7 | 3,646.4 | 1.000 | −0.06 | −0.1 | 8.2 | −18325.4 | 0.959 | −0.07 | 0.4 | 1.4 | 1,147.7 | 0.887 | −0.08 | |
Urea | 1374.6 | 128.3 | 26.4 | 0.007 | 2.33 | 1,108.5 | 115.7 | 29.5 | 0.021 | 1.95 | 527.3 | 77.5 | 41.6 | 0.461 | 0.79 | 424.5 | 387.6 | 258.2 | 0.434 | 0.62 | 322.8 | 84.3 | 73.9 | 0.838 | 0.48 | |
Polyamines and creatine | Creatine | 7.2 | 1.3 | 51.9 | 0.373 | 0.43 | 7.8 | 1.4 | 50.2 | 0.425 | 0.47 | 0.4 | 0.8 | 551.1 | 0.928 | 0.05 | 4.6 | 7.9 | 484.0 | 0.632 | 0.28 | 1.9 | 0.8 | 118.8 | 0.858 | 0.10 |
Creatinine | 13.8 | 1.4 | 27.7 | 0.115 | 1.13 | 10.6 | 1.0 | 27.2 | 0.126 | 0.83 | 2.6 | 0.8 | 87.5 | 0.869 | 0.20 | 7.0 | 5.1 | 206.5 | 0.365 | 0.51 | 2.4 | 1.4 | 161.6 | 0.858 | 0.18 | |
Pyruvate metabolism | Lactate | 1285.8 | 90.8 | 20.0 | 0.002 | 2.91 | 1129.1 | 55.3 | 13.8 | 0.008 | 2.60 | 535.6 | 76.4 | 40.3 | 0.593 | 1.07 | 976.5 | 266.9 | 77.3 | 0.087 | 1.75 | 623.1 | 57.5 | 26.1 | 0.499 | 1.25 |
Pyruvate | −17.4 | 8.0 | −130.9 | 0.332 | −0.82 | −8.5 | 4.3 | −143.8 | 0.549 | −0.44 | −38.2 | 5.4 | −39.6 | 0.148 | −1.44 | 66.2 | 10.0 | 42.7 | 0.004 | 7.60 | −4.5 | 3.4 | −210.7 | 0.935 | −0.16 | |
Short-chain fatty acids (SCFAs) | Acetate | −1.0 | 2.5 | −718.5 | 0.815 | −0.12 | −18.8 | 2.0 | −29.5 | 0.031 | −1.66 | −22.5 | 2.9 | −36.6 | 0.078 | −1.85 | −13.6 | 5.3 | −110.7 | 0.343 | −1.15 | −5.1 | 1.8 | −100.1 | 0.858 | −0.40 |
Butyrate | 1.4 | 0.2 | 35.5 | 0.031 | 1.85 | 0.9 | 0.2 | 70.0 | 0.126 | 1.07 | 0.4 | 0.1 | 97.2 | 0.781 | 0.45 | −0.5 | 0.5 | −290.0 | 0.632 | −0.45 | 0.2 | 0.3 | 314.2 | 0.858 | 0.29 | |
Formate | −123.1 | 2.0 | −4.5 | 0.002 | −20.91 | −24.7 | 0.6 | −6.5 | 0.002 | −9.27 | −171.4 | 2.6 | −4.3 | 0.004 | −23.60 | −1.3 | 0.7 | −144.7 | 0.506 | −0.65 | −1.2 | 0.5 | −120.6 | 0.858 | −0.64 | |
Sugars | Glucose | −18253.0 | 338.5 | −5.2 | 0.002 | −27.52 | 377.6 | 48.4 | 36.2 | 0.039 | 1.22 | −200.2 | 74.0 | −104.6 | 0.869 | -0.47 | 6.7 | 150.7 | 6,328.0 | 0.955 | 0.04 | 6.9 | 69.9 | 2,858.2 | 1.000 | 0.02 |
Mannose | 5.3 | 1.3 | 68.5 | 0.293 | 0.76 | 1.4 | 0.8 | 154.8 | 0.878 | 0.20 | −1.7 | 1.4 | −243.3 | 0.879 | −0.26 | −1.8 | 3.4 | −547.7 | 0.768 | −0.18 | −1.9 | 0.9 | −137.4 | 0.858 | −0.25 | |
Myo inositol | 7.2 | 0.7 | 26.7 | 0.003 | 2.75 | 7.3 | 1.0 | 40.1 | 0.002 | 2.97 | 2.6 | 1.2 | 127.3 | 0.461 | 0.98 | 6.7 | 1.1 | 48.1 | 0.010 | 2.33 | 1.7 | 0.5 | 88.0 | 0.838 | 0.62 | |
Tricarboxylic acid (TCA) cycle | 2-Oxoglutarate | 2.4 | 0.7 | 80.0 | 0.096 | 1.16 | 1.2 | 0.7 | 156.7 | 0.373 | 0.52 | −0.7 | 0.7 | −260.8 | 0.869 | −0.35 | 2.6 | 1.5 | 164.6 | 0.191 | 1.07 | 0.6 | 0.3 | 134.1 | 0.858 | 0.24 |
Citrate | −32701.4 | 1,031.2 | −8.9 | 0.002 | −25.64 | −20904.7 | 566.8 | −7.7 | 0.002 | −23.90 | −7.7 | 4.4 | −160.0 | 0.831 | −0.26 | −14.9 | 16.8 | -320.5 | 0.365 | −0.44 | 19.5 | 3.7 | 53.4 | 0.812 | 0.64 | |
Succinate | −2.7 | 0.5 | −50.7 | 0.065 | −1.35 | −0.1 | 0.2 | −587.7 | 0.851 | −0.05 | 0.4 | 0.3 | 208.1 | 1.000 | 0.12 | 1.3 | 1.0 | 221.8 | 0.632 | 0.55 | 0.8 | 0.2 | 87.9 | 0.858 | 0.30 |
Pairwise comparison between serum (Reference) compared to each plasma type was performed using the Mann-Whitney U test.
Effect size (δ) between serum and each plasma tube are presented: |δ| < 0.33 corresponds to small, |δ| < 0.474 corresponds to medium, and |δ| > 0.475 corresponds to large effect size in metabolite concentration differences.