Table 2. Kinetic pKa Values for Wild-Type Enzymes and Mutants Obtained from Fits of the pH-Rate Dataa.
enzyme | pKa1 | pKa2 |
---|---|---|
WT PTP1B | 5.08 ± 0.20 | 6.44 ± 0.26 |
PTP1B T177G | 5.44 ± 0.37 | 6.37 ± 0.28 |
WT YopH | 5.02 ± 0.27 | 5.58 ± 0.34 |
YopH G352T | 4.06 ± 0.23 | 5.70 ± 0.24 |
The pKa1 value arises from the cysteine nucleophile and pKa2 from the aspartic acid.