Skip to main content
. 2021 Aug 3;11:15749. doi: 10.1038/s41598-021-94922-x

Table 2.

Predicted and measured yields in kBq.

Product 82.8 MeV 28Si on natCr 72.0 MeV 16O on natCu 55.0 MeV 16O on natCu
14,400 s 98 pnA 1500 s 111 pnA 1200 s 8.4 pnA
Predicted Measured Predicted Measured Predicted Measured
77Kr 805 4380 ± 170 1281a  < LODa 44.7 51.5 ± 0.04
77Br 38.1 71.9 ± 15 9.21a/37.7b 5.0 ± 1.4a 0.33 1.0 ± 0.5
76Kr 17.9 31.7 ± 3.2 139 18.9 ± 4.5 1.05 0.95 ± 0.3
76Br 17.3 16.7 ± 1.7 134 34.6 ± 3.5 1.74 2.1 ± 1.4

aFor the 72 MeV 16O experiment, counting did not begin until approximately 18 h EOB. Consequentially, any 77Kr produced would have decayed to a level too low to be detected prior to gamma spectroscopy beginning. The measured 77Br therefore represents both directly produced 77Br and the product of 77Kr decay. For both isotopes, the predicted activities are for physical yield at EOB (using the same delivered current profile as the actual irradiation). The effects of simulation error on the predicted yields are negligible compared to variations in delivered beam and are ignored.

bThe 37.7 kBq of 77Br represents the predicted EOB activity that would be found if all 77Kr produced was allowed to decay to 77Br, and then an EOB activity for 77Br was determined by backfitting the decay from that point forward without decay-correcting for 77Kr feeding.