Heralded spectroscopy.
(a) Two-dimensional histogram of photon
pairs following the same excitation pulse, according to the energy
of the first (EBX) and second (E1X) photons (vertical and horizontal axes, respectively),
over a 5 min measurement. Dashed green line serves as a guide to the
eye, marking the same energy for both photons (undetectable by the
system). (b) Spectrum of the BX (red dots), 1X (blue rings), and all
on state detections (gray area, normalized). Solid red and dashed
blue lines are fits of the BX and 1X spectra, respectively, to a Cauchy–Lorentz
distribution. Binding energy, estimated as the difference between
BX and 1X spectral peaks, is εb = 9.3 ± 1.0
meV. (c) Binding energy as a function of 1X spectral peak for 30 QDs.
Error bars depict 68% confidence intervals.