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. 2021 Sep 13;118(38):e2102881118. doi: 10.1073/pnas.2102881118

Fig. 4.

Fig. 4.

Numerical verification of Eq. 10. The blue boundary marks the location of the inequality Tr[A]2Det[A] for a two dimensional square matrix A. The red diamonds are results from the nonequilibrium KMC simulations with the parameters used in Fig. 2 and the red line is the theoretical mean-field prediction for those same parameters. Gray dots are computed by constructing the matrices δμ, D, and L1 using the the master equation results and computing the eigenvalues of (δμDL1)/Jtot using Mathematica (47) for randomly selected parameters from Lβ,eq=[1,90,000], fdensity,β=[1,100], and kgrow=[0.001,100] nm/s, with all other parameters the same as the red line. Inset shows these two quantities for a wider range, with both axes on logarithmic scales. We do not consider kgrow<0.001 nm/s due to limitations of numerical precision. Eq. 1/Eq. 10 provides strong constraints between the nonequilibrium forcing, morphology, and speed of growth.