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Effects of electrostatic interactions on metal-oxido and -hydroxido complexes. Addition of LAn+ accelerates the rate of electron transfer for [FeIV(O)(N4Py)]2+ by up to 108-fold (A). [(15c5)⊃LAII-(μ-OH)-FeIIIMST]+ (LA = Ca, Sr) (B). The previously characterized [(TMC)FeIV–O–ScIII(OTf)4(OH)] was reformulated as [(TMC)FeIII–O–ScIII(OTf)4(OH2)] (C).
