Sticker clustering tunes intradroplet organization.
(A) Assortativity,
a measure of the spatial mixing between stickers and spacers, is measured
for the entire system as a function of sticker strength, spacer strength,
and sticker clustering. For each system, the phase boundary is shown
as a dashed line for reference. For the well-clustered sequences,
significant deviations from a value of 0 are observed. (B) To understand
the origins of these large assortativity values, we generated snapshots
from distinct regions in panel A (orange beads are stickers, and black
beads spacers). These revealed the intradroplet organization of stickers
into local clusters and subdomains. For sequences with the most well-clustered
stickers, we observe an assortativity of >0 at subsaturating concentrations
due to the presence of small labile clusters.