|
|
Concentration (mol m−3) |
|
|
Mean value of (mol m−3) |
|
|
Membrane coefficient based on the Knudsen diffusion model (mol m−2 Pa−1 s−1) |
|
|
Membrane coefficient based on the molecular diffusion model (kg m−2 Pa−1 s−1) |
|
|
Membrane permeation coefficient (mol m−2 Pa−1 s−1) |
|
|
Diffusion coefficient of CO2 in MEA (m2 s−1) |
|
|
Equivalent hydraulic diameter of channel (m), i = spiral, empty |
|
|
Accuracy deviation of experimental results from the theoretical predictions |
|
|
absorption flux enhancement |
|
|
Fanning friction factor |
|
|
Dimensionless Henry’s constant |
|
|
Hydraulic dissipate energy (J kg−1), i = spiral, empty |
|
|
Absorption flux enhancement |
|
|
Power consumption relative index |
|
|
Molar flux (mol m−2 s−1) |
|
|
Mass-transfer coefficient in the gas feed stream (m s−1) |
|
|
Mass-transfer coefficient in the liquid absorbent side (m s−1) |
|
|
Equilibrium constant |
|
|
Reduced equilibrium constant |
|
|
Overall mass-transfer coefficient of membrane (m s−1) |
|
|
Friction loss (J kg−1), j = CO2, MEA |
|
|
Channel length (m) |
|
|
Length of spiral wired channel (m) |
|
|
Average molecular weight of CO2 and N2 gas mixture (kg mol−1) |
|
Nexp
|
Number of experimental measurements |
|
|
Saturation vapor pressure in the gas feed flow side (Pa) |
|
|
Saturation vapor pressure in the liquid absorbent flow side (Pa) |
|
|
Volumetric flow rate of the gas feed stream (m3 s−1) |
|
|
Volumetric flow rate of the MEA absorbent side (m3 s−1) |
|
|
Gas constant (8.314 J mol−1 K−1) |
|
Re
|
Reynolds number |
|
|
Radius of inner tube (m) |
|
|
Radius of shell (m) |
|
rp
|
Membrane pore radius (m) |
|
Sc
|
Dimensionless Schmidt number |
|
ShS
|
Enhanced dimensionless Sherwood number |
|
|
Dimensionless Sherwood number for laminar flow |
|
Wp
|
Pitch width (m) |
|
|
Absorption flux (mol m−2 s−1) |
|
|
Natural log mean CO2 mole fraction in the membrane |
|
|
Axial coordinate along the flow direction (m) |
|
Greek letters
|
|
|
|
Mass-transfer enhancement factor |
|
|
Aspect ratio of the channel |
|
|
Thickness of membrane (µm) |
|
|
Membrane porosity |
|
|
Average velocity (m s−1) |
|
|
Density (kg m−3), i = CO2, MEA |
|
|
Concentration polarization coefficients |
|
Subscripts
|
|
| 1 |
Membrane surface on MEA side |
|
|
Liquid phase on membrane surface on MEA side |
|
|
Gas phase on membrane surface on MEA side |
|
a
|
The gas feed flow channel |
|
b
|
The liquid absorbent flow channel |
|
cal
|
Calculated results |
|
spiral
|
Inserting spiral wires as promoters |
|
empty
|
Empty channel |
|
exp
|
Experimental results |
|
in
|
Inlet |
|
out
|
Outlet |
|
theo
|
Theoretical predictions |
|
Superscripts
|
|
|
con
|
Concurrent-flow operations |
| counter |
Countercurrent-flow operations |