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. 2021 Dec 21;12(1):365–377. doi: 10.1039/d1ra08192f

Computed hyperpolarizability from the two-level model (βtl in ×10−33 esu), change in dipole moment (Δμ in au), excitation energy (ΔE in eV), oscillator strength (fo in au) hyper Rayleigh scattering (βHRS in ×10−33 esu), and depolarization ratio (DR in au) of superalkali clusters.

Superalkalis β tl Δμ ΔE f o β HRS DR
Ge 5 AM 3
Ge5Li3 (A) 1.03 × 10−29 1.05 2.16 0.05 1.31 × 10−29 6.87
Ge5Na3 (B) 3.11 × 10−29 1.14 1.67 0.04 4.23 × 10−29 5.61
Ge5K3 (C) 9.79 × 10−29 2.34 1.58 0.16 1.32 × 10−28 6.41
Ge 9 AM 5
Ge9Li5 (D) 2.90 × 10−30 0.62 1.69 0.01 1.13 × 10−29 2.44
Ge9Na5 (E) 1.90 × 10−27 2.49 0.01 0.002 9.61 × 10−27 2.41
Ge9K5 (F) 9.83 × 10−28 1.86 0.75 0.06 5.03 × 10−26 2.45
Ge 10 AM 3
Ge10Li3 (G) 1.54 × 10−30 0.62 1.87 0.01 1.21 × 10−29 2.37
Ge10Na3 (H) 1.79 × 10−30 0.65 2.02 0.21 2.08 × 10−29 2.45
Ge10K3 (I) 9.64 × 10−31 0.49 1.86 0.11 2.73 × 10−29 2.57