Table 3. Components of the Evolution of the Transverse Magnetization at MHz^a.

	R⊥ (1/s)	1/4(4Δ2 – J1,1 (ω0)2)1/2 (1000/s)	1/8[L1,1(ω0) + 2L2,2(2ω0)] (1/s)
1st h.l. all	0.86 ± 0.01		0.038 ± 0.003
1st h.l., intra	0.46 ± 0.01		0.021–0.003+0.004
1st h.l., inter	0.229 ± 0.002		0.0065 ± 0.0001
1st h.l., pept. H	0.186 ± 0.002		0.0150 ± 0.0005
2nd h.l. all	0.361 ± 0.004		0.0056 ± 0.0004
2nd h.l., intra	0.169–0.002+0.003		0.0013–0.0001+0.0002
2nd h.l., inter	0.1757–0.0010+0.0009		0.00358 ± 0.00005
2nd h.l., pept. H	0.0202–0.0004+0.0005		0.00176–0.00010+0.00014
water intra	0.1469 ± 0.0007	0.8 ± 0.1	0.00087 ± 0.00002
water inter	0.1044–0.0002+0.0003	4.7 ± 0.1	0.001611 ± 0.000009
water, pept. H	0.00598 ± 0.00007	7.82 ± 0.08	0.00054 ± 0.00002

^aErrors represent 95% confidence intervals computed with the bootstrap method. See section 4.1 for an explanation of the labels. The oscillation factor ¹/₄(4Δ² – J_1,1 (ω₀)²)^1/2 is reported only for all water molecules, since the same secular RDC values (Δ/3) were used for the analysis of the hydration layers. See section 4.1 for discussion.