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. 2022 May 16;12:8016. doi: 10.1038/s41598-022-11882-6

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© The Author(s) 2022

Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.

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(a,b) Normalized exciton absorption intensity for three (a) 4.5 and (b) 5.5 ML CQW samples as a function of photogenerated sheet density. Each data point is extracted from a transient absorption spectrum collected at 3 ps pump-probe delay for many powers of 2.72 eV and 3.50 eV pump light. (c,d) Ratio of heavy hole and light hole bleach signals as a function of photogenerated sheet densities for the same (c) 4.5 and (d) 5.5 ML samples. (e,f) Half-width at half-maximum (HWHM) of the HH bleach feature from the transient absorption spectrum (ΔA) plotted against photogenerated sheet densities of the same (e) 4.5 and (f) 5.5 ML samples. In all cases, data for measurements with 3.50 eV pump are shown in solid symbols and data for 2.72 eV pump measurements are shown in open symbols. A solid line represents a smoothed average of 3.50 eV pump experiments and a dashed line corresponds to the smoothed average of 2.72 eV pump.