Table 2.
fac-Ir(ppy)3 | [Ir(dFppy)2dtbbpy]PF6 | fac-Ir(dFppy)3 | |
---|---|---|---|
yield of [2+2]a | 71% | 41% | 49% |
ET (kcal/mol)b | 55.2 | 55.4 | 60.1 |
KSV (4a) (M−1) | 120.8 | 232.1 | 999.7 |
KSV (1) (M−1) | 9.0 | 67.1 | 476.8 |
KSV (4a) /KSV (1) | 13.4 | 3.5 | 2.1 |
Condition: 4a (0.2 mmol, 1.0 equiv), 1 (5.0 equiv), [Ir] (1.0 mol %) in CH2Cl2 (0.4 M), 450 nm, 24 h.
ref. (27)