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. 2022 Aug 29;17(9):2643–2654. doi: 10.1021/acschembio.2c00575

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© 2022 The Authors. Published by American Chemical Society

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Time-dependent evolution of TRIR bands. (A) Kinetic traces of the excited state decay (1384 cm^–1) and the ground-state recovery (1546 cm^–1, shown inverted for comparison). (B) Comparison of the rise and decay of radical intermediates in wild-type OaPAC. (C) Comparison of the rise and decay of radical transient at 1528 cm^–1 with transient evolving at 1635 cm^–1. (D) Kinetic trace of the 1694 cm^–1 transient, assigned to light-state formation. Raw data are shown as solid lines or dots, while global fitting results are shown as dashed lines.