| [Ni(NCS)2(C6H7N)4]·2C2H3N | F(000) = 1320 |
| Mr = 629.48 | Dx = 1.249 Mg m−3 |
| Monoclinic, C2/c | Cu Kα radiation, λ = 1.54184 Å |
| a = 18.7990 (1) Å | Cell parameters from 26840 reflections |
| b = 11.3033 (1) Å | θ = 4.5–79.2° |
| c = 15.8639 (1) Å | µ = 2.25 mm−1 |
| β = 96.825 (1)° | T = 100 K |
| V = 3347.04 (4) Å3 | Block, light purple |
| Z = 4 | 0.25 × 0.15 × 0.05 mm |