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. 2022 Nov 22;61(51):e202214610. doi: 10.1002/anie.202214610

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© 2022 The Authors. Angewandte Chemie International Edition published by Wiley-VCH GmbH

This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc-nd/4.0/ License, which permits use and distribution in any medium, provided the original work is properly cited, the use is non‐commercial and no modifications or adaptations are made.

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A) AetF‐catalyzed aromatic iodination and cycloiodoetherification. Conversions were determined from relative integration values for starting material and product for reactions conducted on 75 μL scale; selected isolated yields (isol.) and assay yields (AY) relative to authentic internal standards were also obtained for reactions conducted on 20–30 mL scale. B) Bromination and iodination of tryptophan catalyzed by AetF (red and orange traces, respectively) and AetF K258A (blue traces), showing no conversion to either halogenated product using the latter enzyme. GDH=glucose dehydrogenase, Cat.=catalase.