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. 2023 Jan 10;14:146. doi: 10.1038/s41467-022-35667-7

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© The Author(s) 2023

Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

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Fig. 1 — a Formation of thick SCL when uncoated NMC811 is in direct contact with a sulfide SSE; b reduced SCL with an oxide coating on NMC811; and c a gradient lithium oxide-oxy-thiophosphate interface tailoring a smooth transition from oxide-favored to sulfide-favored. d Schematic representation of an NMC811 primary particle (pink colour) with an ionic conductive and gradient Li₃P_1+xO₄S_4x coating (blue colour). SCL stands for space-charge layer and PS-LPO-NMC stands for gradient Li₃P_1+xO₄S_4x-coated NMC811.