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. 2023 Jan 10;127(3):1560–1575. doi: 10.1021/acs.jpcc.2c05103

Table 4. Unit Cell Parameters for MIL-68(Al) and MIL-53(Al) Obtained via Energy Minimization (opt) and Averaging over the MD Trajectory (avg.) at SCC DFTB and GFN2-xTB Level in Comparison to the Experimental Reference Data.

system cell size parameter set kmax a b c
MIL-68(Al) 1·1·3 avg. matsci 1 21.200 35.988 6.769
avg. matsci 0 21.195 35.979 6.769
avg. GFN2 1 20.251 33.201 6.606
opt. matsci 1 21.227 36.066 6.792
opt. matsci 0 21.217 36.082 6.806
opt. GFN2 1 21.037 34.971 6.638
exp.74   20.51(1) 35.92(1) 6.683(1)
             
MIL-53(Al) 2·1·1 avg. matsci 1 6.767 16.787 12.992
avg. matsci 0 6.766 16.803 12.970
avg. GFN2 1 6.458 17.222 11.319
opt. matsci 1 6.789 16.853 12.945
opt. matsci 0 6.804 16.500 13.408
opt. GFN2 1 6.730 17.710 10.964
exp. 548 K68   6.608(1) 16.675(3) 12.813(2)