aReactions were performed with 7.5 MBq [77Br]bromide, 1 μmol of boronic pinacol ester precursor, 0.5 μmol of [Cu(py)4(OTf)2], and 3,4,7,8-Tetramethyl-1,10-phenanthroline (Ligand) stirred in 100 μL of 9:1 MeOH::H2O for 30 minutes at room temperature (rt). bAll reactions were conducted in duplicate and RCC calculated as activity trapped on C18 cartridge versus starting activity scaled by HPLC radioactivity detector chromatogram product peak area versus all peak areas to account for impurities.